首页|3D-Printing Functional Ceramic for One-Step Fabrication of Pd/C Catalytic Reactor

3D-Printing Functional Ceramic for One-Step Fabrication of Pd/C Catalytic Reactor

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Catalysts are widely used in the chemical industry because of their environmental friendliness and low energy consumption.However,integrated fabrication of catalytic reactors(CRs)remains challenging.In this study,we propose the integrated manufacturing of a palladium-carbon(Pd/C)CR for the first time.The outer shell ink com-prises Al2O3 powder and aluminum dihydrogen phosphate(AP),whereas the inner core ink consists of activated carbon powder,AP,and polymethylmethacrylate(PMMA).By integrating with the coaxial 3D printing strategy,the Pd/C CR can be freeform-designed with different core thicknesses,lengths,and shapes(W-type,L-type,and U-type).Based on this,a CR with excellent catalytic properties was further developed by loading palladium(Pd)particles.Typically,the resultant Pd/C CR with a length of 2.5 cm exhibits a catalytic efficiency of up to 97.6%after 60 min.This method of preparing Pd/C CR using coaxial 3D printing combines multimaterial 3D print-ing,integrated molding,and complex biomimetic structure fabrication.This offers a feasible and cost-effective solution that uses a simple fabrication process.

Coaxial 3D printingCatalytic reactorPalladium-carbon catalystCatalytic reduction

Shengcai Wu、Xin Xu、Xiaotong Zhang、Zhongying Ji、Xin Jia、Xiaolong Wang

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School of Chemistry and Chemical Engineering/State Key Laboratory Incubation Base for Green Processing of Chemical Engineering,Shihezi University,Shihezi,832003,China

State Key Laboratory of Solid Lubrication,Lanzhou Institute of Chemical Physics,Chinese Academy of Sciences,Lanzhou,730000,China

Shandong Laboratory of Advanced Materials and Green Manufacturing at Yantai,Yantai Zhongke Research Institute of Advanced Materials and Green Chemical Engineering,Yantai,264006,China

2024

中国机械工程学报:增材制造前沿(英文)