首页|Enhanced visible light absorption of Bi2WO6/SiO2 with abundant adsorbed oxygen for the degradation of organic pollutant

Enhanced visible light absorption of Bi2WO6/SiO2 with abundant adsorbed oxygen for the degradation of organic pollutant

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Heterogeneous photocatalysts exhibit high catalytic efficiency in the degradation of pollutants,but their stability and repeatability is not very good and requires high structural matching.Simply by nanosizing the pure Bi2WO6(BWO)photocatalyst without constructing a heterojunction,there is a significant improvement in its performance,with an enhancement effect of about 2.3 times(99.43%).The high photocatalytic degradation efficiency of the material can be attributed to the enhanced light absorption effect brought by the three-dimensional inverse-opal structure SiO2(IS)and the abundant surface adsorbed oxygen generated after the formation of Si-O-W bonds.In addition,the introduction of IS greatly increases the surface area of nanostructured BWO,which accelerates the charge transfer process,while the adsorbed oxygen promotes the participation of·O2-in the photocatalytic reaction,thereby accelerating the consumption of photo-generated electrons and ultimately improving the separation of charge carriers.Furthermore,the matched photonic bandgap further improves the absorption and uti-lization of light of the material.In this work,we constructs Si-O-W bonds to obtain inverse-opal SiO2/Bi2WO6 with uniformly growth of pure phase nano BWO,which provides a feasible strategy for the preparation of high-performance pure-phase photocatalysts.

Bi2WO6SiO2 inverse-opal structurePhotocatalysisAdsorbed oxygen

Yuanting Wu、Xiaoying Wang、Wenlong Zhong、Shan Zhang

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School of Material Science and Engineering,Shaanxi University of Science and Technology,Xi'an 710021,China

国家自然科学基金Youth Innovation Team of Shaanxi Universities

521732142022-70

2024

颗粒学报(英文版)
中国颗粒学会 中国科学院过程工程研究所

颗粒学报(英文版)

CSTPCD
影响因子:0.632
ISSN:1674-2001
年,卷(期):2024.88(5)
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