电催化还原二氧化碳合成C3+产物

Steering electroreduction of carbon dioxide to valuable C3+products

罗雨婷 ¹胡书萁 ²刘碧录²

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作者信息

1. Department of Electrical and Computer Engineering,University of Toronto,Toronto,Ontario M5S 3G4,Canada
2. Shenzhen Geim Graphene Center,Shenzhen Key Laboratory of Layered Materials for Value-Added Applications,Tsinghua-Berkeley Shenzhen Institute &Institute of Materials Research,Tsinghua Shenzhen International Graduate School,Tsinghua University,Shenzhen 518055,China
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摘要

通过电催化还原反应将二氧化碳(CO2)转换为重要燃料和化工原料意义重大,有利于推进工业低碳化发展.如今,该技术路线可以实现C1和C2产物的高选择性、快速合成,但合成高值碳三加(C3+)产物的转化率仍较低.本文中,我们聚焦电催化还原二氧化碳合成C3+产物的进展,重点关注CO2转化为C3+产物的催化剂材料、电化学系统和串联反应器这三个方面.最后,本文指出了该领域面临的主要挑战和未来的研究方向.

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基金项目

National Science Foundation of China for Distinguished Young Scholars(52125309)

National Natural Science Foundation of China(52188101)

Guangdong Basic and Applied Basic Research Foundation(2022B1515120004)

Guangdong Innovative and Entrepreneurial Research Team Program(2017ZT07C341)

Innovation Team Project of the Department of Education of Guangdong Province(2023KCXTD051)

Shenzhen Basic Research Project(WDZC20220812141108001)

Tsinghua Shenzhen International Graduate School-Shenzhen Pengrui Young Faculty Program of Shenzhen Pengrui Foundation(SZPR2023002)

Banting Postdoctoral Fellowships Program(01353-000)

出版年

2024

中国科学:材料科学(英文)

CSTPCD

ISSN：

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