首页|Photophysics of metal-organic frameworks:A brief overview

Photophysics of metal-organic frameworks:A brief overview

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Metal-organic frameworks(MOFs),which are self-assembled porous coordination materials,have garnered consid-erable attention in the fields of optoelectronics,photovoltaic,photochemistry,and photocatalysis due to their diverse struc-tures and excellent tunability.However,the performance of MOF-based optoelectronic applications currently falls short of the industry benchmark.To enhance the performance of MOF materials,it is imperative to undertake comprehensive investigations aimed at gaining a deeper understanding of photophysics and sequentially optimizing properties related to photocarrier transport,recombination,interaction,and transfer.By utilizing femtosecond laser pulses to excite MOFs,time-resolved optical spectroscopy offers a means to observe and characterize these ultrafast microscopic processes.This approach adds the time coordinate as a novel dimension for comprehending the interaction between light and MOFs.Ac-cordingly,this review provides a comprehensive overview of the recent advancements in the photophysics of MOFs and additionally outlines potential avenues for exploring the time domain in the investigation of MOFs.

metal-organic framework(MOF)ultrafast spectroscopyphotophysicscarrier dynamics

刘晴硕、余俊宏、胡建波

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State Key Laboratory for Environment-Friendly Energy Materials,Southwest University of Science and Technology,Mianyang 621010,China

Laboratory for Shock Wave and Detonation Physics,Institute of Fluid Physics,China Academy of Engineering Physics,Mianyang 621900,China

Science Challenge ProjectNational Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaProject of State Key Laboratory of Environmentfriendly Energy Materials,and Southwest University of Science and Technology

TZ2018001118720582180203621fksy07

2024

10.1088/1674-1056/acfe00

中国物理B(英文版)
中国物理学会和中国科学院物理研究所

中国物理B(英文版)

CSTPCDEI
影响因子：0.995
ISSN：1674-1056
年,卷(期)：2024.33(1)
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