首页|Single crystal growth and characterization of 166-type magnetic kagome metals

Single crystal growth and characterization of 166-type magnetic kagome metals

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Kagome magnets were predicted to be a good platform to investigate correlated topology band structure,Chern quantum phase,and geometrical frustration due to their unique lattice geometry.Here we reported single crystal growth of 166-type kagome magnetic materials,including HfMn6Sn6,ZrMn6Sn6,GdMn6Sn6 and GdV6Sn6,by using the flux method with Sn as the flux.Among them,HfMn6Sn6 and ZrMn6Sn6 single crystals were grown for the first time.X-ray diffraction measurements reveal that all four samples crystallize in HfFe6Ge6-type hexagonal structure with space group P6/mmm.All samples show metallic behavior from temperature dependence of resistivity measurements,and the dom-inant carrier is hole,except for GdV6Sn6 which is electron dominated.All samples have magnetic order with different transition temperatures,HfMn6Sn6,ZrMn6Sn6 and GdV6Sn6 are antiferromagnetic with TN of 541 K,466 K and 4 K respectively,while GdMn6Sn6 is ferrimagnetic with the critical temperature of about 470 K.This study will enrich the research platform of magnetic kagome materials and help explore the novel quantum phenomena in these interesting mate-rials.The dataset of specific crystal structure parameters for HfMn6Sn6 are available in Science Data Bank,with the link https://doi.org/10.57760/sciencedb.j00113.00120.

kagome metalsingle crystal growthcrystal structurephysical property

吴黄宇、刘锦锦、李永恺、朱鹏、杨柳、陈富红、胡灯、王秩伟

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Centre for Quantum Physics,Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurement(MOE),School of Physics,Beijing Institute of Technology,Beijing 100081,China

Beijing Key Laboratory of Nanophotonics and Ultra fine Optoelectronic Systems,Beijing Institute of Technology,Beijing 100081,China

Material Science Center,Yangtze Delta Region Academy of Beijing Institute of Technology,Jiaxing 314011,China

Beijing Institute of Technology,Zhuhai 519000,China

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Beijing Natural Science FoundationNational Key Research and Development Program of ChinaNational Key Research and Development Program of ChinaBeijing National Laboratory for Condensed Matter Physics

Z2100062022YFA14034002020YFA03088002023BNL-CMPKF007

2024

中国物理B(英文版)
中国物理学会和中国科学院物理研究所

中国物理B(英文版)

CSTPCDEI
影响因子:0.995
ISSN:1674-1056
年,卷(期):2024.33(9)