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Chiral polaritons in semiconductor perovskite metasurface enhanced by bound states in the continuum

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Chiral polaritons in semiconductor perovskite metasurface enhanced by bound states in the continuum
The exploration of novel chiral optical platforms holds both fundamental and practical importances,which have shown great promise towards applications in valleytronics,chiral sensing and nanoscopic chiroptics.In this work,we combine two key concepts—chiral bound states in the continuum and exciton polaritons—to showcase a strong chiral response from polaritons.Using the finite element method,we numerically design a CsPbBr3 based metasurface that supports intrinsically chiral bound states in the continuum and verify the chirality by calculating the reflection spectrum and eigen-polarization mapping.We further demonstrate chirality-dependent exciton polariton angular dispersion arising from the strong coupling between the chiral BIC and excitons in CsPbBr3 by simulating the polariton angle-resolved absorption spectrum.Reciprocity analysis reveals that the polariton photoluminescence in different momentum space locations is selectively enhanced by chiral pumping light.Our results suggest a promising first step towards chiral polaritonics.

bound states in the continuumchiralitymetasurfaceperovskite microcavitiesexciton polariton

汪顿、Albert Y.Xiong、Julia Q.Zhang、佘增德、康晓峰、朱莹、Sanjib Ghosh、熊启华

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State Key Laboratory of Low-Dimensional Quantum Physics,Department of Physics,Tsinghua University,Beijing 100084,China

Tsinghua International School,Beijing 100084,China

Beijing Academy of Quantum Information Sciences,Beijing 100193,China

Frontier Science Center for Quantum Information,Beijing 100084,China

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bound states in the continuum chirality metasurface perovskite microcavities exciton polariton

2024

中国物理B(英文版)
中国物理学会和中国科学院物理研究所

中国物理B(英文版)

CSTPCDEI
影响因子:0.995
ISSN:1674-1056
年,卷(期):2024.33(12)