首页|Interception of Layered LP-N and HLP-N at Ambient Conditions by Confined Template
Interception of Layered LP-N and HLP-N at Ambient Conditions by Confined Template
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We propose a feasible strategy of intercepting the layered polymeric nitrogen(LP-N)and hexagonal layered polymeric nitrogen(HLP-N)at ambient conditions by using the confinement templates.The stable mechanism of confined LP-N and HLP-N at ambient conditions is revealed,namely the synergistic effect of charge transfer and vdW confinement effect.The influence rule of interlayer spacing on the stability of LP-N is revealed.Most importantly,the nitrogen content and energy density of recoverable LP-N@graphene(70.59％,8.15kJ/g),LP-N@h-BN(70.59％,7.96 kJ/g),HLP-N@graphene(68.97％,9.31 kJ/g),and HLP-N@h-BN(69.57％,8.05 kJ/g)refresh the new record for the confinement polynitrogen system.
王冬雪、付静、李义、姚震、刘爽、刘冰冰
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State Key Laboratory of Superhard Materials,College of Physics,Jilin University,Changchun 130012,China
Basic Science Department,Jilin Institute of Architecture and Technology,Changchun 130000,China
College of Science,Liaoning University of Technology,Jinzhou 121000,China
国家重点研发计划国家自然科学基金国家自然科学基金Natural Science Foundation Project of Liaoning Province
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