首页|Giant Magneto-Optical Effect in van der Waals Room-Temperature Ferromagnet Fe3GaTe2

Giant Magneto-Optical Effect in van der Waals Room-Temperature Ferromagnet Fe3GaTe2

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The discovery of ferromagnetic two-dimensional(2D)van der Waals(vdWs)materials provides an opportu-nity to explore intriguing physics and to develop innovative spin electronic devices.However,the main challenge for practical applications of vdWs ferromagnetic crystals lies in the weak intrinsic ferromagnetism and small per-pendicular magnetic anisotropy(PMA)above room temperature.Here,we report the intrinsic vdWs ferromag-netic crystal Fe3GaTe2,synthesized by the self-flux method,exhibiting a Curie temperature(TC)of 370K,a high saturation magnetization of 33.47 emu/g,and a large PMA energy density of approximately 4.17 × 105 J/m3.Fur-thermore,the magneto-optical effect is systematically investigated in Fe3GaTe2.The doubly degenerate E2g(Γ)mode reverses the helicity of incident photons,indicating the existence of pseudoangular-momentum(PAM)and chirality.Meanwhile,the non-degenerate non-chiral A1g(Γ)phonon exhibits a significant magneto-Raman effect under an external out-of-plane magnetic field.These results lay the groundwork for studying phonon chirality and magneto-optical phenomena in 2D magnetic materials,providing the feasibility for further fundamental research and applications in spintronic devices.

张晓敏、王健、朱文凯、张佳茜、李伟浩、张菁、王开友

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State Key Laboratory of Superlattices and Microstructures,Institute of Semiconductors,Chinese Academy of Sciences,Beijing 100083,China

Center of Materials Science and Optoelectronics Engineering,University of Chinese Academy of Sciences,Beijing 100049,China

School of Materials,Shenzhen Campus of Sun Yat-sen University,Shenzhen 518107,China

National Key Research and Development Program of ChinaBeijing Natural Science Foundation Key ProgramNational Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaNational Natural Science Foundation of China

2022YFA1405100Z220005122414051217438412204058

2024

中国物理快报(英文版)
中国科学院物理研究所,中国物理学会

中国物理快报(英文版)

CSTPCDEI
影响因子:0.515
ISSN:0256-307X
年,卷(期):2024.41(6)