首页|Superior triethylamine-sensing properties based on SnO2 hollow nanospheres synthesized via one-step process

Superior triethylamine-sensing properties based on SnO2 hollow nanospheres synthesized via one-step process

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Due to serious harm of triethylamine(TEA)to environmental safety and human health,it is significant to syn-thesize gas-sensitive materials with high performance for TEA detection.However,it is still a challenge to achieve high-sensitivity detection of TEA at low temperature for a sensor synthesized through an economical and efficient method.In this work,hollow-structured SnO2(HS-SnO2)nanospheres have been fabricated by a facile,low-cost hydrothermal method in one step,which exhibit superior TEA-sensing properties,including not only ultrahigh response(127.75)for 100 ppm TEA,good selectivity,but also fast response and recovery time(17/28 s),low detection threshold(1 ppm)and robust stability at a relatively low optimum operational temperature of 225 ℃.The excellent gas-sensitizing performances are ascribed to porous hollow structures with rich oxygen vacancies that provide abundant active sites for raising O2 adsorption and reaction of TEA and oxygen species.This work offers an effective and economical strategy for fabricating high-performance TEA sensors for industrial applications.

Hollow-structured SnO2 nanospheresTEAHigh responseGas sensors

Mingyue Xu、Shu Yan、Zia Ur Rehman、Jianhua Hou、Liangyun Zhai、Shengjie Zhu、Chuanbao Cao、Wanfeng Xie、Junyu Zhong、Jun Yang

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State Key Laboratory of Bio-fibers and Eco-textiles,School of Electronics and Information,College of Materials Science and Engineering,College of Chemistry and Chemical Engineering,Qingdao University,Qingdao,266071,China

College of Environmental Science and Engineering,Yangzhou University,Yangzhou,Jiangsu,225009,China

State Key Laboratory of Chemical Safety,SINOPEC Research Institute of Safety Engineering Co.,Ltd.,Qingdao,266104,China

National Registration Center for Chemicals,Ministry of Emergency Management Qingdao,266071,China

Research Center of Materials Science,Beijing Institute of Technology,Beijing,100081,China

State Key Laboratory of Multiphase Complex Systems,Institute of Process Engineering,Chinese Academy of Sciences,Beijing,100190,China

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2024

自然科学进展·国际材料(英文)
国家自然科学基金委员会

自然科学进展·国际材料(英文)

影响因子:0.25
ISSN:1002-0071
年,卷(期):2024.34(4)