首页|硫-铁自养反硝化人工湿地强化农村黑臭水体深度脱氮

硫-铁自养反硝化人工湿地强化农村黑臭水体深度脱氮

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现阶段研究分析发现,N、S元素是导致水体黑臭的关键所在,由此构建硫-铁自养反硝化人工湿地系统治理农村黑臭水体.该自养反硝化系统以硫铁矿为电子供体、以青石为酸碱平衡调节材料,按照3∶2、1∶1的比例混合,通过分析不同水力停留时间(HRT)下湿地系统的脱氮效果、沿程脱氮变化及微生物群落情况,验证该人工湿地系统的脱氮治理效果.结果表明,在HRT为24 h条件下系统的脱氮效果最好,TN、NO-3-N分别从(12.88±0.4)、(7.73±0.76)mg/L降至(1.46±0.34)、(0.83±0.14)mg/L,最高去除率分别为91.3%、91.8%;但随着HRT的下降,脱氮效果也随之降低.随取样口1~4相对高度的增加,系统脱氮效率明显上升,其中,由硫铁矿、火山岩、青石按照3∶5∶2的体积比复配而成的人工湿地系统在取样口4的TN及NO-3-N去除率分别为87.07%、85.88%,取样口1的TN及NO-3-N去除率仅为15.91%、16.88%.此外,Proteobacteria(变形门菌)、Bacteroidetes(拟杆菌门)等为该系统中的优势菌门.
Effect of Sulfur-iron Autotrophic Denitrification Constructed Wetland on Nitrogen in Black and Smelly Water
Current studies indicated that N and S elements were the key factors leading to water body black and odor. A S-Fe self-supporting denitrifying wetland system was constructed to control the black and odor water in rural areas of the Yellow River Basin. The autotrophical denitrification system used py-rite as electron donor and bluestone as acid-base balance regulating material,mixed at ratios of 3∶2 and 1∶1. The nitrogen removal effect of the constructed wetland system with different hydraulic residence time (HRT),the change in nitrogen removal along the path and microbial communities,were analyzed to verify the nitrogen removal and treatment effect of the constructed wetland system. The results showed that the system had the best denitrification effect when HRT was 24 h. TN and NO-3-N decreased from (12.88±0.4),(7.73±0.76) mg/L to (1.46±0.34) and (0.83±0.14) mg/L respectively,with the highest removal rates of 91.3% and 91.8%. However,with the decrease of HRT,the nitrogen removal effect decreased. With the increase of relative height of sampling port 1~4,the nitrogen removal efficien-cy of the system increased significantly. Among them,the TN and NO-3-N removal rates of the construc-ted wetland system composed of pyrite,volcanic rock and bluestone with the volume ratio of 3∶5∶2,at the sampling port 4 were 87.07% and 85.88%,respectively. The removal rates of TN and NO-3-N of sampling port 1 were only 15.91% and 16.88%. In addition,Proteobacteria and Bacteroidetes were the dominant bacteria in this system.

rural dark smelling water bodiesautotrophic denitrificationconstructed wetlandsdenitrifcation effectalong course changes

高镜清、李煜翾、张政、王世龙、王帅、张鑫

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郑州大学生态与环境学院 河南郑州 450001

水利部黄河流域水治理与水安全重点实验室 河南郑州 450003

中建八局华中建设有限公司 湖北武汉 430021

河海大学环境学院 江苏南京 210098

郑州源致和环保科技有限公司 河南郑州 450001

广州铁诚工程质量检测有限公司 广东广州 510010

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农村黑臭水体 自养反硝化 人工湿地 脱氮效果 沿程变化

2025

郑州大学学报(理学版)
郑州大学

郑州大学学报(理学版)

北大核心
影响因子:0.437
ISSN:1671-6841
年,卷(期):2025.57(2)