首页|A superhydrophobic Fe3O4@MSN-PDMS based composite coating with icephobicity, long-term durability and self-healing property for anti-/de-icing

A superhydrophobic Fe3O4@MSN-PDMS based composite coating with icephobicity, long-term durability and self-healing property for anti-/de-icing

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  • NETL
  • NSTL
  • Elsevier
© 2024 Elsevier LtdIce formation is a ubiquitous phenomenon in various fields and often leads to catastrophic consequences. Despite numerous anti-icing coating strategies have been exploited, there are still multiple roadblocks in the way of developing anti-icing coatings with durable and effective anti-/de-icing properties. In this work, Fe3O4 was coated in-situ with mesoporous silica nanoparticle (MSN), in which a high dosage of polydimethylsiloxane (PDMS) was then loaded. As-obtained core-shelled Fe3O4@MSN-PDMS aggregates were incorporated into silicone resin to construct an NIR responsive anti-/de-icing coating via spraying method. The as-prepared coating exhibited superhydrophobicity (156.7° of water contact angle) and delayed icing time to 412 s under −20 °C. Besides, the prepared coating could heat and release PDMS to constitute a PDMS/water double-layer lubricant under NIR irradiation, significantly reducing ice adhesion strength from 90.60 kPa to 12.04 kPa. Furthermore, the prepared coating demonstrates self-healing properties and high durability, releasing PDMS stored in the coating sustainably to heal the damaged coating surface and keeping superhydrophobicity after chemical etching and mechanical erosion. Finally, the de-icing applicability of the coating was validated using a homemade rotor wing model. Such core-shelled anti-/de-icing materials would provide a theoretical basis and a brand-new design strategy for development and application of anti-/de-icing materials.

Anti-icing coatingPhotothermal de-icingRotor wingSelf-healing

Deng L.、Wang Z.、Yu H.、Li Y.、Cao Y.、Luo F.、Chen Q.、Wu J.、Gu X.、Liu X.

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State Key Laboratory of Solidification Processing School of Materials Science and Engineering Northwestern Polytechnical University

State Key Laboratory of Solidification Processing School of Materials Science and Engineering Northwestern Polytechnical University||Key laboratory of Materials Processing and Mold Zhengzhou University

AVIC Xi'an Aircraft Industry (Group) Company Ltd.

Key Laboratory of Icing and Anti/De-icing of China Aerodynamics Research and Development Center

Key laboratory of Materials Processing and Mold Zhengzhou University

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2025

10.1016/j.compscitech.2024.110937

Composites science and technology

Composites science and technology

SCI
ISSN：0266-3538
年,卷(期)：2025.259(Jan.5)
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