首页|Development of cinnamaldehyde/aminated gelatin film as pH-responsive controlled-release packaging for cherry preservation: Effects of CO_2 and humidity in the microenvironment

Development of cinnamaldehyde/aminated gelatin film as pH-responsive controlled-release packaging for cherry preservation: Effects of CO_2 and humidity in the microenvironment

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pH-responsive materials control the release of active substances by responding to pH changes in the environment.In this study, based on the properties of imine bond with acid-sensitive hydrolysis and mild reactionconditions, cinnamaldehyde was immobilized onto aminated gelatin (AGel) films to generate cinnamaldehyde/aminated gelatin (Cin/AGel) films, which were then applied to preserve cherries. FTIR and XPS confirmed thesynthesis of imine bonds. The excellent pH-responsive controlled-release properties of Cin/AGel films weredemonstrated by monitoring changes in the cumulative release fraction of cinnamaldehyde in the aqueous phase(different pH buffers) and in atmospheric environments (different CO_2 concentrations and humidity). Even whennot in direct contact with the aqueous phase, it can nevertheless provide effective regulated release to theacidified environment caused by CO_2 accumulation and high humidity conditions. Furthermore, the Cin/AGelfilms had smart antibacterial properties. Compared to PE and AGel films, Cin/AGel film packaging increased theshelf life of cherries by 9 and 6 days at 4 ℃, respectively. As a result, the shown pH-responsive controlled-releasefilms have promising applications in controlling the release of antimicrobial agents during food preservation.

PH-responsiveImine bondsCinnamaldehydeSmart food packagingCherries preservation

Xianhui Tang、Meiyan Zhu、Ling Zhang、Liang Zhu

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College of Food Science and Engineering, South China University of Technology, Guangdong 510640, China

College of Biological and Food Engineering, Guangdong University of Petrochemical Technology, Maoming, China

2025

Food Packaging and Shelf Life

Food Packaging and Shelf Life

ISSN:
年,卷(期):2025.48(1)
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