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Europium diffusion in IG-110 nuclear graphite

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Europium diffusion in graphite has been recognized to be of interest in high-temperature gas reactor safety analysis, particularly as an indicator of strontium diffusion. However, no measurements of europium diffusion coefficients have been reported in the literature. In this work, the effective diffusion coefficient of europium was measured using a time-release method. Natural europium was loaded into pre milled unirradiated IG-110 graphite spheres using a pressurized acid digestion vessel. The time-release experiments were performed in the temperature range 1823 K - 1973 K using a SiC diffusion cell connected to an inductively-coupled plasma mass spectrometer (ICP-MS) via a He gas line. The results of this work are:& nbsp;D-Eu, IG-110 = (1 . 5 x 10(-3)m(2)/(s))exp(-2 . 87 x10(5) J/mol /RT ) This effective diffusion coefficient can be used to aid in predictive modelling of europium transport in HTGRs. (C)& nbsp;2022 Elsevier B.V. All rights reserved.

IG-110GraphiteEuropiumDiffusion coefficientHTGRICP-MS MEASUREMENTMETALLIC FISSION-PRODUCTSRELEASE BEHAVIORFUEL COMPACTSCOEFFICIENTSPARTICLESIODINECESIUM

Weilert, T. M.、Walton, K. L.、Loyalka, S. K.、Brockman, J. D.

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Univ Missouri

2022

Journal of Nuclear Materials

Journal of Nuclear Materials

EISCI
ISSN:0022-3115
年,卷(期):2022.561
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