首页|Facile synthesis of highly dispersed Ru/functionalized CMK-3 catalyst with superior catalytic wet air oxidation (CWAO) performance of ammonia

Facile synthesis of highly dispersed Ru/functionalized CMK-3 catalyst with superior catalytic wet air oxidation (CWAO) performance of ammonia

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This article proposes a novel decamethonium bromide (DATB)-assisted hydrothermal method to synthesize highly dispersed Ru/functionalized CMK-3 catalyst for catalytic wet air oxidation (CWAO) of ammonia. The proposed strategy anchors RuCl62- onto the electropositive DAT (decyltrimethylammonium ion)-modified CMK3-N support. As a consequence, the aggregation of Ru nanoparticles during high temperature treatment is inhibited by the electrostatic interaction between the Ru species and CMK-3-N-DTA as well as the isolation effect of carbon deposits. The DMH-AH catalyst exhibits superior activity and selectivity for ammonia nitrogen removal than the reference catalyst synthesized via traditional impregnation method.

Ammonia-containing wastewaterCatalytic wet air oxidationRu-based catalystHigh dispersionBIMETALLIC RU-CUWASTE-WATERTRANSITION-METALSIMULTANEOUS REMOVALCARBONNANOPARTICLESINSIGHTSNITROGENTOXICITYKINETICS

Gai, Hengjun、Li, Donghui、Song, Hongbing、Zhao, Xixi、Xiao, Meng、Zhu, Quanhong、Huang, Tingting

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Qingdao Univ Sci & Technol

2022

Chemical Physics Letters

Chemical Physics Letters

EISCI
ISSN:0009-2614
年,卷(期):2022.793
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