Applied Catalysis2022,Vol.3129.DOI:10.1016/j.apcatb.2022.121422

Triboelectric pulsed direct-current enhanced radical generation for efficient degradation of organic pollutants in wastewater

Liu, Xinliang Mo, Jilong Wu, Wanhai Song, Hainong Nie, Shuangxi
Applied Catalysis2022,Vol.3129.DOI:10.1016/j.apcatb.2022.121422

Triboelectric pulsed direct-current enhanced radical generation for efficient degradation of organic pollutants in wastewater

Liu, Xinliang 1Mo, Jilong 1Wu, Wanhai 1Song, Hainong 2Nie, Shuangxi1
扫码查看

作者信息

  • 1. Guangxi Univ
  • 2. Guangxi Bossco Environm Protecting Technol Co Ltd
  • 折叠

Abstract

The generation of free radicals was enhanced by triboelectric pulsed direct-current during the organic pollutant degradation. The self-powered electrochemical system was constructed for enhancing 4-CP removal powered by a water-driven triboelectric nanogenerator (WD-TENG). The output of current, voltage, and power of WD-TENG were studied. The removal of 4-CP and its degradation mechanism were also discussed. The results shows that the formation of hydroxyl radicals (center dot OH) was improved by improving PMA(Mo5+) conversion efficiency by the WD-TENG in the phosphomolybdic acid/H2O2 (PMA/H2O2) system, resulting the mineralizing the 4-CP via dichlorination and oxidation. The removal of 4-CP improved by 10% in 120 min in the WD-TENG powered electro-PMA/H2O2 system. This study provides a promising methodology for improving the performance of self-powered electrochemical processes for the treatment of environmental pollution.

Key words

Triboelectric nanogenerator/Radical generation/Pulsed direct-current/4-chlorophenol/Waste water treatment/ELECTRO-FENTON DEGRADATION/ADVANCED OXIDATION PROCESSES/CARBON MATERIALS/REMOVAL/4-CHLOROPHENOL/NANOGENERATOR/SYSTEM/ACID

引用本文复制引用

出版年

2022
Applied Catalysis

Applied Catalysis

ISSN:0926-3373
被引量23
参考文献量61
段落导航相关论文