首页|Preparation of highly dispersed Pt/Hp catalyst via supercritical fluid deposition and its catalytic performance for combustion of toluene
Preparation of highly dispersed Pt/Hp catalyst via supercritical fluid deposition and its catalytic performance for combustion of toluene
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NSTL
The emission of volatile organic compounds (VOCs) causes serious atmospheric environmental problems and catalytic combustion is one of the most promising methods in the treatment of VOCs. In this work, the Pt/Hp catalyst was fabricated via supercritical fluid deposition (SFD) for the first time and its activity was evaluated for toluene catalytic combustion. The preparation conditions during the SFD process were optimized. Na2PtCl6 was selected as the precursor and 450 °C as the reduction temperature. The catalysts prepared by the SFD and impregnation (IM) were compared. The Pt/Hp catalyst prepared by SFD had smaller size and higher dispersion and its T90 was 25 °C lower than that prepared by IM, which showed obvious size effect. For the similar activity, the Pt loading on catalyst prepared by SFD is only 50% of that on catalyst prepared by IM, showing obvious reduction effect for noble metal.
Key Laboratory for Green Chemical Technology of Ministry of Education, R&D Center for Petrochemical Technology, Tianjin University, Tianjin, 300072, China
NSTL
