首页|(163022)Enhanced performance of solution-processed all-inorganic halide perovskite photodetectors by using bulk heterojunction and lateral configuration

(163022)Enhanced performance of solution-processed all-inorganic halide perovskite photodetectors by using bulk heterojunction and lateral configuration

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Currently, ail-inorganic halide perovskites are widely investigated for their applications in optoelectronics due to their excellent physical and chemical properties. In this paper, solution-processed bulk-hetero-junction lateral photodetectors Ag/CsPbBr_3:ZnO/Ag were built to enhance device performance, in which the active CsPbBr_3 layer were surface-passivated by ZnO nanoparticles (NPs) in an optimized molar ratio. By optimizing the molar ratio of CsPbBr_3 to ZnO NPs (i.e. fcR=M_(CsPbBr_3)/M_(ZnO)). the photocurrent from the lateral photodetector was greatly enhanced and, the dark current was suppressed to as low as 10~(12) A due to the lateral configuration by employing a 50 pm-width active layer made through an interdigital mask. As a result, the On/Off current ratio of the lateral photodetector Ag/CsPbBr_3:ZnO/Ag reaches to more than 10~3 for an optimum molar ratio k_R= 1:1, and it is 300-folds higher than that of the control device Ag/CsPbBr_3/Ag, showing a maximum specific detectivity D* of 1.6 × 10~(11) Jones with a photoresponsivity of 3.8 mA/W under 16 pW/cm~2 405 nm illumination at - 5 V. In this way, it provides an efficient method for solution-processed high-performance photodetectors by combining bulk heterojunction and lateral configuration.

Bulk heterojunctionSolution-processedLateral photodetectorAll-inorganic halide perovskitesZnO nanoparticles (NPs)

Peiyun Tang、Shengyi Yang、Jinming Hu

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Beijing Key Laboratory of Nanophotonics and Ultrafine Optoelectronic Systems, School of Physics, Beijing Institute of Technology, Beijing 100081, PR China

2022

Journal of Alloys and Compounds

Journal of Alloys and Compounds

EISCI
ISSN:0925-8388
年,卷(期):2022.896
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