首页|One-pot synthesis of nanosized MnO incorporated into N-doped carbon nanosheets for high performance lithium storage

One-pot synthesis of nanosized MnO incorporated into N-doped carbon nanosheets for high performance lithium storage

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As potential anode materials for lithium-ion batteries, transition metal oxides have been extensively investigated due to their high theoretical capacity. Nevertheless, how to address rapid capacity degradation and improve rate capability is still a big challenge. Herein, nanosized MnO incorporated into N-doped carbon nanosheets (MnO/NCN) was rationally designed by a facile one-pot salt-templated synthesis method. The nanosized MnO particles (around 20 nm) were powerfully anchored on the ultrathin N-doped carbon nanosheets to build a high-efficiency electrons/ions hybrid conductive framework. In addition, based on the stable interfacial interaction between MnO and N-doped carbon nanosheets, the MnO/NCN hybrid exhibits great structural stability, thus delivering high reversible lithium storage capacity (719 mA h g?1 at 0.1 A g?1) and superior stability (497 mA h g?1 at 1 A g?1 over 1000 cycles). Besides, the assembled lithium-ion capacitor with MnO/NCN anode exhibits excellent energy-power characteristics (142 W h kg?1 at 412 W kg?1). Such impressive lithium storage performance demonstrates that the MnO/NCN electrode is promising for large-scale energy storage devices.

Anode materialsLithium-ion batteriesLithium-ion capacitorsN-doped carbonNanosized MnO

Sun Z.、Liu C.、Shi J.、Huang M.、Liu S.、Shi Z.、Wang H.

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School of Materials Science and Engineering Ocean University of China

2022

Journal of Alloys and Compounds

Journal of Alloys and Compounds

EISCI
ISSN:0925-8388
年,卷(期):2022.902
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