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纳微快报(英文)
安徽省地质学会
纳微快报(英文)

安徽省地质学会

月刊

2311-6706

liyingzhang@sjtu.edu.cn

021-34207624

200240

上海市闵行区东川路800号

纳微快报(英文)/Journal Nano-Micro LettersCSCDCSTPCD北大核心EISCI
查看更多>>Nano-Micro Letters《纳微快报(英文)》是上海交通大学主办、在Springer Nature开放获取出版的英文学术期刊,主要报道纳米/微米尺度相关的高水平文章(research article, review, communication, perspective, highlight, etc),包括:微纳米材料与结构的合成表征与性能及其在能源、催化、环境、传感、电磁波吸收与屏蔽、生物医学等领域的应用研究。期刊已被SCI、EI、SCOPUS、PubMed Central、DOAJ、CSCD、知网、万方、维普、超星等数据库收录。JCR学科排名在物理、材料、纳米学科领域均位于Q1区,入选了中科院期刊分区材料科学1区TOP期刊。Nano-Micro Letters《纳微快报(英文)》先后入选“中国科技期刊国际影响力提升计划D类(2013年)和B类(2016-2018年)”,上海市高水平高校学术期刊支持计划A类(2016-2021年),“上海交通大学学术期刊影响力提升计划A类(2019年)”等。曾荣获中国出版政府奖期刊提名奖(2021年),中国最具国际影响力学术期刊奖(2015-2021年),中国高校杰出科技期刊(2018、2020年),华东地区优秀期刊(2021年),华东地区期刊优秀栏目(2020年),上海市高校精品科技期刊奖(2016、2018、2020年),上海市期刊编校质量优秀奖(2019年),中国高校百佳科技期刊(2016年),中国高校科技期刊优秀网站(2017年)等。
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    Scalable Ir-Doped NiFe2O4/TiO2 Heterojunction Anode for Decentralized Saline Wastewater Treatment and H2 Production

    Sukhwa HongJiseon KimJaebeom ParkSunmi Im...
    1-18页
    查看更多>>摘要:Wastewater electrolysis cells(WECs)for decentralized wastewater treatment/reuse coupled with H2 production can reduce the carbon footprint associated with transportation of water,waste,and energy carrier.This study reports Ir-doped NiFe2O4(NFI,~5 at%Ir)spinel layer with TiO2 overlayer(NFI/TiO2),as a scalable heterojunction anode for direct electrolysis of wastewater with circum-neutral pH in a single-compartment cell.In dilute(0.1 M)NaCl solutions,the NFI/TiO2 marks superior activity and selectivity for chlorine evolution reaction,outperforming the benchmark IrO2.Robust operation in near-neutral pH was confirmed.Electroanalyses including operando X-ray absorption spectroscopy unveiled crucial roles of TiO2 which serves both as the primary site for Cl-chemisorption and a protective layer for NFI as an ohmic contact.Galvanostatic electrolysis of NH4+-laden synthetic wastewater demonstrated that NFI/TiO2 not only achieves quasi-stoichiometric NH4+-to-N2 conversion,but also enhances H2 generation efficiency with minimal competing reactions such as reduction of dissolved oxygen and reactive chlorine.The scaled-up WEC with NFI/TiO2 was demonstrated for electrolysis of toilet wastewater.

    Inter-Skeleton Conductive Routes Tuning Multifunctional Conductive Foam for Electromagnetic Interference Shielding,Sensing and Thermal Management

    Xufeng LiChunyan ChenZhenyang LiPeng Yi...
    19-36页
    查看更多>>摘要:Conductive polymer foam(CPF)with excellent compressibility and variable resistance has promising applications in electromagnetic interfer-ence(EMI)shielding and other integrated functions for wearable electronics.However,its insufficient change amplitude of resistance with compressive strain generally leads to a degradation of shielding performance during deformation.Here,an innovative loading strategy of conductive materials on polymer foam is proposed to significantly increase the contact probability and contact area of con-ductive components under compression.Unique inter-skeleton conductive films are constructed by loading alginate-decorated magnetic liquid metal on the poly-methacrylate films hanged between the foam skeleton(denoted as AMLM-PM foam).Traditional point contact between conductive skeletons under compression is upgraded to planar contact between conductive films.Therefore,the resistance change of AMLM-PM reaches four orders of magnitude under compression.Moreover,the inter-skeleton conductive films can improve the mechanical strength of foam,prevent the leakage of liquid metal and increase the scattering area of EM wave.AMLM-PM foam has strain-adaptive EMI shielding performance and shows compression-enhanced shielding effec-tiveness,solving the problem of traditional CPFs upon compression.The upgrade of resistance response also enables foam to achieve sensitive pressure sensing over a wide pressure range and compression-regulated Joule heating function.

    Multifunctional Nacre-Like Nanocomposite Papers for Electromagnetic Interference Shielding via Heterocyclic Aramid/MXene Template-Assisted In-Situ Polypyrrole Assembly

    Jinhua XiongXu ZhaoZonglin LiuHe Chen...
    37-54页
    查看更多>>摘要:Robust,ultra-flexible,and multifunctional MXene-based electromagnetic interference(EMI)shielding nanocomposite films exhibit enormous potential for applications in artificial intelligence,wireless telecommunication,and portable/wearable electronic equip-ment.In this work,a nacre-inspired multifunctional heterocyclic aramid(HA)/MXene@polypyrrole(PPy)(HMP)nanocomposite paper with large-scale,high strength,super toughness,and excellent tolerance to complex conditions is fabricated through the strategy of HA/MXene hydrogel template-assisted in-situ assembly of PPy.Benefiting from the"brick-and-mortar"layered structure and the strong hydrogen-bonding interactions among MXene,HA,and PPy,the paper exhibits remarkable mechanical performances,including high tensile strength(309.7 MPa),outstanding toughness(57.6 MJ m-3),exceptional foldability,and structural stability against ultrasonication.By using the template effect of HA/MXene to guide the assembly of conductive polymers,the synthesized paper obtains excellent electronic conductivity.More importantly,the highly continuous conductive path enables the nanocomposite paper to achieve a splendid EMI shielding effectiveness(EMI SE)of 54.1 dB at an ultra-thin thickness(25.4 μm)and a high specific EMI SE of 17,204.7 dB cm2 g-1.In addition,the papers also have excellent applications in electromagnetic protection,electro-/photothermal de-icing,thermal therapy,and fire safety.These findings broaden the ideas for developing high-performance and multifunctional MXene-based films with enormous application potentialin EMI shielding and thermal management.

    Smart Gas Sensors:Recent Developments and Future Prospective

    Boyang ZongShufang WuYuehong YangQiuju Li...
    55-86页
    查看更多>>摘要:Gas sensor is an indispensable part of modern society with wide applications in environmental monitoring,healthcare,food industry,public safety,etc.With the development of sensor technology,wireless com-munication,smart monitoring terminal,cloud storage/computing technol-ogy,and artificial intelligence,smart gas sensors represent the future of gas sensing due to their merits of real-time multifunctional monitoring,early warning function,and intelligent and automated feature.Various electronic and optoelectronic gas sensors have been developed for high-performance smart gas analysis.With the development of smart terminals and the maturity of integrated technology,flexible and wearable gas sensors play an increas-ing role in gas analysis.This review highlights recent advances of smart gas sensors in diverse applications.The structural components and fundamental principles of electronic and optoelectronic gas sensors are described,and flexible and wearable gas sensor devices are highlighted.Moreover,sensor array with artificial intelligence algorithms and smart gas sensors in"Internet of Things"paradigm are introduced.Finally,the challenges and perspectives of smart gas sensors are discussed regarding the future need of gas sensors for smart city and healthy living.

    Defect Engineering with Rational Dopants Modulation for High-Temperature Energy Harvesting in Lead-Free Piezoceramics

    Kaibiao XiJianzhe GuoMupeng ZhengMankang Zhu...
    87-101页
    查看更多>>摘要:High temperature piezoelectric energy harvester(HT-PEH)is an important solution to replace chemical battery to achieve independent power supply of HT wireless sensors.However,simultane-ously excellent performances,including high figure of merit(FOM),insulation resistivity(ρ)and depolarization temperature(Td)are indis-pensable but hard to achieve in lead-free piezoceramics,especially oper-ating at 250℃ has not been reported before.Herein,well-balanced performances are achieved in BiFeO3-BaTiO3 ceramics via innovative defect engineering with respect to delicate manganese doping.Due to the synergistic effect of enhancing electrostrictive coefficient by polariza-tion configuration optimization,regulating iron ion oxidation state by high valence manganese ion and stabilizing domain orientation by defect dipole,comprehensive excellent electrical performances(Td=340℃,P250 ℃>107 Ω cm and FOM250 ℃=4905×10-15 m2 N-1)are realized at the solid solubility limit of manganese ions.The HT-PEHs assembled using the rationally designed piezoceramic can allow for fast charging of commercial electrolytic capacitor at 250℃ with high energy conversion efficiency(η=11.43%).These characteristics demonstrate that defect engineering tailored BF-BT can satisfy high-end HT-PEHs requirements,paving a new way in developing self-powered wireless sensors working in HT environments.

    Wafer-Scale Vertical 1D GaN Nanorods/2D MoS2/PEDOT∶PSS for Piezophototronic Effect-Enhanced Self-Powered Flexible Photodetectors

    Xin TangHongsheng JiangZhengliang LinXuan Wang...
    102-116页
    查看更多>>摘要:van der Waals(vdW)heterostructures constructed by low-dimensional(0D,1D,and 2D)materials are emerging as one of the most appealing systems in next-generation flexible photodetection.Currently,hand-stacked vdW-type photodetectors are not compatible with large-area-array fabrication and show unimpressive performance in self-powered mode.Herein,vertical 1D GaN nanorods arrays(NRAs)/2D MoS2/PEDOT∶PSS in wafer scale have been proposed for self-powered flexible photodetectors arrays firstly.The as-integrated device without external bias under weak UV illumination exhibits a competitive responsivity of 1.47 A W-1 and a high detectivity of 1.2×1011 Jones,as well as a fast response speed of 54/71 μs,thanks to the strong light absorption of GaN NRAs and the efficient photogenerated carrier separation in type-Ⅱ heterojunction.Notably,the strain-tunable photodetection performances of device have been demonstrated.Impressively,the device at-0.78%strain and zero bias reveals a significantly enhanced photoresponse with a responsivity of 2.47 A W-1,a detectivity of 2.6×1011 Jones,and response times of 40/45 μs,which are superior to the state-of-the-art self-powered flexible photodetectors.This work presents a valuable avenue to prepare tunable vdWs heterostructures for self-powered flexible photodetection,which performs well in flexible sensors.

    Laser-Induced Highly Stable Conductive Hydrogels for Robust Bioelectronics

    Yibo LiHao ZhouHuayong YangKaichen Xu...
    117-120页
    查看更多>>摘要:Despite the promising progress in conductive hydrogels made with pure con-ducting polymer,great challenges remain in the interface adhesion and robustness in long-term monitoring.To address these challenges,Prof.Seung Hwan Ko and Taek-Soo Kim's team introduced a laser-induced phase separation and adhesion method for fabricating conductive hydrogels consisting of pure poly(3,4-ethylenedioxythiophene):polystyrene sulfonate on polymer substrates.The laser-induced phase separation and adhesion treated conducting polymers can be selectively transformed into conductive hydrogels that exhibit wet conductivities of 101.4 S cm-1 with a spatial resolution down to 5 μm.Moreover,they maintain impedance and charge-storage capacity even after l h of sonication.The micropatterned electrode arrays demonstrate their potential in long-term in vivo signal record-ings,highlighting their promising role in the field of bioelectronics.

    Electrode/Electrolyte Optimization-Induced Double-Layered Architecture for High-Performance Aqueous Zinc-(Dual)Halogen Batteries

    Chengwang ZhouZhezheng DingShengzhe YingHao Jiang...
    121-137页
    查看更多>>摘要:Aqueous zinc-halogen batteries are promising candidates for large-scale energy storage due to their abundant resources,intrinsic safety,and high theoretical capacity.Nevertheless,the uncontrollable zinc dendrite growth and spontaneous shuttle effect of active species have prohibited their practical implementation.Herein,a double-layered protective film based on zinc-ethylenediamine tetramethylene phospho-nic acid(ZEA)artificial film and ZnF2-rich solid electrolyte interphase(SEI)layer has been successfully fabricated on the zinc metal anode via electrode/electrolyte synergistic optimization.The ZEA-based artificial film shows strong affinity for the ZnF2-rich SEIlayer,therefore effec-tively suppressing the SEI breakage and facilitating the construction of double-layered protective film on the zinc metal anode.Such double-layered architecture not only modulates Zn2+flux and suppresses the zinc dendrite growth,but also blocks the direct contact between the metal anode and electrolyte,thus mitigating the corrosion from the active species.When employing optimized metal anodes and electrolytes,the as-developed zinc-(dual)halogen batteries present high areal capacity and satisfactory cycling stability.This work provides a new avenue for developing aqueous zinc-(dual)halogen batteries.

    Nanograting-Based Dynamic Structural Colors Using Heterogeneous Materials

    Jingang WangHaibo YuJianchen ZhengYuzhao Zhang...
    138-151页
    查看更多>>摘要:Dynamic structural colors can change in response to different environmental stimuli.This ability remains effective even when the size of the species responsible for the structural color is reduced to a few micrometers,providing a promising sensing mechanism for solving microen-vironmental sensing problems in micro-robotics and microfluid-ics.However,the lack of dynamic structural colors that can encode rapidly,easily integrate,and accu-rately reflect changes in physical quantities hinders their use in microscale sensing applications.Herein,we present a 2.5-dimensional dynamic structural color based on nanogratings of heterogeneous materials,which were obtained by interweaving a pH-responsive hydrogel with an IP-L photoresist.Transverse gratings printed with pH-responsive hydrogels elongated the period of longitudinal grating in the swollen state,resulting in pH-tuned structural colors at a 45°incidence.Moreover,the patterned encoding and array printing of dynamic structural colors were achieved using grayscale stripe images to accurately encode the periods and heights of the nanogrid structures.Overall,dynamic structural color networks exhibit promising potential for applications in information encryption and in situ sensing for microfluidic chips.

    Ideal Bi-Based Hybrid Anode Material for Ultrafast Charging of Sodium-Ion Batteries at Extremely Low Temperatures

    Jie BaiJian Hui JiaYu WangChun Cheng Yang...
    152-167页
    查看更多>>摘要:Sodium-ion batteries have emerged as competitive sub-stitutes for low-temperature applications due to severe capacity loss and safety concerns of lithium-ion batteries at-20℃ or lower.However,the key capability of ultrafast charging at ultralow temperature for SIBs is rarely reported.Herein,a hybrid of Bi nanoparticles embedded in car-bon nanorods is demonstrated as an ideal material to address this issue,which is synthesized via a high temperature shock method.Such a hybrid shows an unprecedented rate performance(237.9 mAh g-1 at 2 A g-1)at-60℃,outperforming all reported SIB anode materials.Coupled with a Na3V2(PO4)3 cathode,the energy density of the full cell can reach to 181.9 Wh kg-1 at-40℃.Based on this work,a novel strategy of high-rate activation is proposed to enhance performances of Bi-based materials in cryogenic conditions by creating new active sites for interfacial reaction under large current.