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天然水体中总α和总β放射性来源分析

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天然水放射性源自溶于水中的放射性核素.总α和总β放射性能够反映各类水体放射性总体水平,是水质辐射监测的筛选指标.原生放射性核素如铀系、钍系衰变系列核素和独立长寿命核素40 K等是天然水放射性的主要来源;238 U、235 U和232Th三个天然衰变系以α衰变为主,β衰变只占小部分;40K的β衰变过程常常是水中总β放射性的主要贡献者.20余种宇生放射性核素中除了3H和14C以外,其他浓度都很低,干湿沉降作用和光合作用可以使3H和14C迁移进入地球圈层并进入天然水中.遇酸遇热不稳定的、易挥发的、半衰期短的放射性核素不能被低本底测量方法有效测定,没有呈现在最终的表观总α和总β活度浓度结果中.单一放射性核素的测量需要采用特定的采样保存技术和分析方法.
Analysis of the origination of gross α and gross β in natural waters
Natural water radioactivity was derived from radionuclides dissolved in water.Gross α and gross β radioactivity can reflect the overall radioactive level in various water bodies andwerescreening indicators for water quality radiation monito-ring.Primordial radionuclides such as uranium,thorium decay series nuclides and independent long-lived nuclide 40K were-the major sources of natural water radioactivity.α decay dominates in the three natural decay series of 238 U,235 U and 232 Th,and β decay was only a small part.The β decay process of 40Kwas usually the main contributor of gross β in natural waters.Except for 3H and 14C,other 20 cosmogenic radionuclides were at low levels.3H and 14C can enter the Earth'sphere through dry and wet deposition and photosynthesis and exist in natural waters.The radionuclides which was unstable to acid and heat,volatile and short half-life cannot be effectively determined by low-background measurement method and were not presented in the final apparent gross radioactive concentration results.The measurement of a single radionuclide requires specific sam-pling and preservation techniques and analytical methods.

natural watersgross αgross βlow-background measurement method

张译文、谢银凤、段明杰、亓恒振

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山东省淄博生态环境监测中心,山东淄博 255000

山东省潍坊生态环境监测中心,山东潍坊 261041

天然水 总α 总β 低本底测量法

2024

地下水
陕西省水工程勘察规划研究院 全国地下水信息网 陕西省水利学会

地下水

影响因子:0.219
ISSN:1004-1184
年,卷(期):2024.46(5)