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人类活动对木里冻土区水文环境影响的多元同位素示踪

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为查明人类活动对木里冻土区水文环境造成的影响,选取高寒冻土区人类活动最为显著的木里煤田聚乎更矿区,以区内大通河支流水系河水为研究对象,基于水化学组成空间特征,利用氢、氧、碳、氮、硫、锶等多元同位素开展示踪研究.研究表明:(1)冻结层上水是河水的主要补给来源,煤矿开采、天然气水合物钻探等人类活动破坏原有冻土结构,增加了冻结层上水对河水的贡献比例;(2)河水中主要溶解性营养物质(SO42-、NO3-和DOC)浓度的增加源于人类活动的影响:硫氧同位素揭示了大规模的煤矿露天开采促进还原硫氧化,是导致冻结层上水和河水中SO42-升高的主要原因;氮氧同位素表明河水中高浓度的NO3-来源于散养式放牧的牲畜粪便;DOC主要来源于高寒草甸植物降解产生的土壤有机质,人类活动影响下增加了DOC和DIC的输出,增强了源区河水中的微生物活动;(3)除H2CO3 风化碳酸盐岩外,受人类活动煤矿开采影响下硫酸参与的碳酸盐岩和硅酸盐岩岩石风化作用增强,进而影响着区域岩石风化的碳汇作用.研究成果为认识人类活动影响下高寒冻土区水文环境的演化提供研究思路,为高寒冻土区生态环境保护提供科学依据.
Multi-Isotope Tracing of the Impact of Human Activities on the Hydrological Environment in the Muli Permafrost Region
In order to find out the impact of human activities on the hydrological environment of Muli permafrost area,Juhugeng mining area of Muli Coalfield with the most significant human activities in the alpine permafrost area was selected,and the river water of Datong River tributary system in the area was taken as the research object.Based on the spatial characteristics of hydrochemical composition,the research was carried out by using multiple isotopes such as hydrogen,oxygen,carbon,nitrogen,sulfur and strontium.The results show that:(1)The supra-permafrost water is the main supply source of the river water.Human activities such as coal mining and natural gas hydrate drilling destroy the original frozen soil structure and increase the contribution proportion of the supra-permafrost water to river water;(2)The increase of the concentration of main dissolved nutrients(SO42-,NO3-and DOC)in river water is due to the influence of human activities:sulfur and oxygen isotopes reveal that large-scale open-pit mining in coal mine promotes reduced sulfur oxidation,which is the main reason for the increase of SO42-in the supra-permafrost water and river water;Nitrogen and oxygen isotopes show that the high concentration of NO3-in the river comes from livestock manure of free range grazing;DOC mainly comes from soil organic matter produced by plant degradation in alpine meadow,and there are strong microbial activities in the river water in the source area;(3)Except for H2CO3 weathering carbonate rocks,the weathering of carbonate rock and silicate rock participated by sulfuric acid is enhanced under the influence of human activities and coal mining,which further affects the carbon sink of regional rock weathering.The research results provide research ideas for understanding the evolution of hydrological environment in Alpine permafrost area under the influence of human activities,and provide scientific basis for ecological environment protection in Alpine permafrost area.

Muli permafrost regioncoal mininggas hydrate drillingisotopesHuman activitieshydrogeology

邢剑伟、李小倩、周爱国、庞守吉、李鑫、余迎祥

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中国地质大学环境学院,湖北武汉 430074

国家环境保护水污染溯源与管控重点实验室,湖北武汉 430074

中国地质调查局油气资源调查中心,北京 100083

木里冻土区 煤矿开采 天然气水合物钻探 同位素 环境效应 水文地质

中国地调局非常规油气地质重点实验室开放基金陆域天然气水合物资源综合调查项目

DD2019137-YQ19JJ02DD20190102

2024

地球科学
中国地质大学

地球科学

CSTPCD北大核心
影响因子:1.447
ISSN:1000-2383
年,卷(期):2024.49(5)
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