首页|Zeolite-confined Fe-site Catalysts for the Hydrogenation of CO2 to Produce High-value Chemicals

Zeolite-confined Fe-site Catalysts for the Hydrogenation of CO2 to Produce High-value Chemicals

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Zeolite-confined Fe-site catalysts(ZFCs)have emerged as superior materials for sustainably producing high-value chemicals through CO2 hydrogenation,owing to their adaptable framework,customizable composition,and thermal robustness.They excel in activating,adsorbing,and converting CO2 with remarkable efficiency and consistency in performance.This has sparked a surge in research interest in recent years.The review delves into the latest advancements in CO2 catalytic hydrogenation to olefins,alcohols,aromatics,and other liquid hydrocarbons,examining the synthesis,modification tactics,and the correlation between structure and performance across various ZFCs.Additionally,it underscores the pivotal factors affecting performance and sheds light on the mechanisms behind selectivity control in the CO2 hydrogenation process facilitated by ZFCs.To conclude,it presents pressing challenges and strategic recommendations to inspire the development of high-performance,durable ZFCs for CO2 hydrogenation applications.

Zeolite-confined Fe-site catalystCO2 hydrogenationModification strategyHigh-value chemical

HAN Xiaoyang、XIA Huicong、TU Weifeng、WEI Yifan、XUE Dongping、LI Minhan、YAN Wenfu、ZHANG Jia-Nan、HAN Yi-Fan

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College of Materials Science and Engineering,Zhengzhou University,Zhengzhou 450001,P.R.China

State Key Laboratory of Coking Coal Resources Green Exploitation,Zhengzhou University,Zhengzhou 450001,P.R.China

Engineering Research Center of Advanced Functional Material Manufacturing of Ministry of Education,School of Chemical Engineering,Zhengzhou University,Zhengzhou 450001,P.R.China

State Key Laboratory of Inorganic Synthesis and Preparative Chemistry and College of Chemistry,Jilin University,Changchun 130012,P.R.China

State Key Laboratory of Chemical Engineering,East China University of Science and Technology,Shanghai 200237,P.R.China

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National Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaScience and Technology R&D Program Joint Fund Project of Henan Province,ChinaDistinguished Young Scholars Innovation Team of Zhengzhou University,ChinaPostgraduate Education Reform Project of Henan Province,ChinaNational Funded Postdoctoral Researcher Program,ChinaKey Research Projects of University in Henan Province,China

U22A20107U19672152207830722208314222783792223800322002008222301420001323202752021SJGLX093YGZC2023238224A150041

2024

10.1007/s40242-023-3269-9

高等学校化学研究(英文版)
吉林大学

高等学校化学研究(英文版)

CSTPCD
影响因子：0.871
ISSN：1005-9040
年,卷(期)：2024.40(1)
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