Progress and Outlook of Carbon-supported Single-atom Electrocatalyst for Oxygen Reduction Reaction

WANG Chengbin ¹LI Ping ¹CHEN Dehong ²ZHANG Ruiyong ³WANG Lei ¹ZONG Lingbo¹

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作者信息

1. College of Chemistry and Molecular Engineering,Qingdao University of Science and Technology,Qingdao 266042,P.R.China
2. College of Materials Science and Engineering,Qingdao University of Science and Technology,Qingdao 266042,P.R.China
3. Key Laboratory of Marine Environmental Corrosion and Bio-fouling,Institute of Oceanology,Chinese Academy of Sciences,Qingdao 266071,P.R.China
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Abstract

Single-atom catalysts(SACs)have garnered extensive attention in the field of catalysis due to their exceptional inherent reaction activity,optimal utilization of metal atoms,etc.Controlled synthesis plays a crucial role in elucidating the structure-activity relationship of SACs.This paper reviews various synthetic strategies for SACs,encompassing defect engineering,metal-organic frameworks(MOFs)pyrolysis,and ion exchange.With specific examples,the significance of constructing catalysts at the atomic level is discussed,aiming to comprehensively understand the synthetic strategies of SACs.Finally,it addresses the challenges and prospects associated with controlled synthesis techniques for SACs as well as their future applications.

Key words

Single-atom catalyst/Synthetic strategy/Carbon support/Oxygen reduction reaction

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基金项目

国家自然科学基金(52172208)

Taishan Scholar Young Talent Program,China(tsqn202306216)

Taishan Scholar Talent Program,China(ts20190402)

出版年

2024

高等学校化学研究(英文版)

吉林大学

高等学校化学研究(英文版)

CSTPCD

影响因子：0.871

ISSN：1005-9040

参考文献量94

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