Recent Advance in Electrocatalytic Water Splitting for Hydrogen Production by Layered Double Hydroxides

XIA Tian ¹REN Qinghui ¹YANG Jiangrong ¹LI Zhenhua ²SHAO Mingfei ²DUAN Xue²

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作者信息

1. State Key Laboratory of Chemical Resource Engineering,College of Chemistry,Beijing University of Chemical Technology,Beijing 100029,P.R.China
2. State Key Laboratory of Chemical Resource Engineering,College of Chemistry,Beijing University of Chemical Technology,Beijing 100029,P.R.China;Quzhou Institute for Innovation in Resource Chemical Engineering,Quzhou 324000,P.R.China
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Abstract

Collecting green hydrogen(H2)from water splitting driven by renewable energy is a new competition to implement the construction of H2 energy industry and promote new economic growth for global governments.The common strategy to enhance the efficiency of H2 production is to reduce the potential of electrolytic cell that is the mainstream way to prepare efficient electrocatalysts.Layered double hydroxides(LDHs)are one of the most active electrocatalysts with adjustable active sites in contemporary research.In this review,we discuss the recent advanced progress of LDHs for hydrogen evolution reaction(HER)on cathode and oxygen evolution reaction(OER)or organic oxidation on anode and emphasize the influence of LDHs structure regulation in water electrolysis process(HER/OER)as well as the current development status of organic oxidation catalyzed by active oxygen species on anode.Finally,we propose the current challenges of LDHs in electrocatalysis and prospect their developing tendency and further application.

Key words

layered double hydroxide/Hydrogen production/Hydrogen evolution reaction(HER)/Oxygen evolution reaction(OER)/Electrocatalytic organic oxidation

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基金项目

National Key Research and Development Program of China(2022YFA1504200)

National Natural Science Foundation of China(22090031)

National Natural Science Foundation of China(22108008)

National Natural Science Foundation of China(22288102)

Young Elite Scientist Sponsorship Program by the China Association for Science and Technology(2021QNRC001)

Fundamental Research Funds for the Central Universities,China(buctrc202011)

出版年

2024

高等学校化学研究(英文版)

吉林大学

高等学校化学研究(英文版)

CSTPCD

影响因子：0.871

ISSN：1005-9040

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