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基于小波变换的湖南省PM2.5污染特征分析

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该文基于湖南省2017-2021年PM2。5与其他5种大气污染物浓度监测数据以及气象资料,分析了 PM2。5浓度时空分布特征,利用连续小波变换和小波相干谱分别研究了 PM2。5浓度周期、PM2。5与其他大气污染物及气象因子的相关性,确定了 PM2。5浓度的主要影响因子,结果表明:(1)湖南省PM2。5浓度年平均值总体呈下降趋势,年均下降率达4。88%,PM2。5浓度月平均值呈"U"型分布,2017年1月月均值浓度最高(91。9 μg/m3),2020年6月月均值浓度最低(15。8 μg/m3);PM2。5浓度年平均值的空间分布则呈现东北至西南高、西北及东南低的特点,PM2。5浓度季平均值呈现冬季>秋季>春季>夏季的特征。(2)14个市(州)PM2。5浓度都存在显著周期性变化,主要包括272 d左右的长周期和36d左右的短周期。(3)PM2。5浓度与其他大气污染物的相关性在不同时频尺度上存在差异。PM2。5浓度与PM10浓度在所有时频尺度上均存在显著的正相关。在小时频尺度(0~64d)上,PM2。5浓度与O3、CO、NO2和SO2浓度都存在正相关性;在中时频尺度(64~256d)上,PM2。5浓度与O3浓度的相关性不明显,与CO、NO2和SO2浓度存在正相关;在大时频尺度(256~512d)上,PM2。5浓度与O3浓度呈现负相关,与NO2和SO2浓度呈现正相关,PM2。5浓度与CO浓度在长沙和衡阳呈现正相关,在怀化呈现负相关。(4)PM2。5浓度与气象因子的相关性在不同时频尺度上也存在差异。在小时频尺度上,PM2。5与降水量、相对湿度和气压存在负相关,与温度和日照时数存在正相关,与风速存在正相关也存在负相关;在中时频尺度上,PM2。5与各气象因子的相关性均不明显;在大时频尺度上,PM2。5与降水、温度和日照时数呈现负相关,PM2。5与气压呈现正相关,PM2。5与相对湿度和风速的相关性不明显。
Analysis of PM2.5 Pollution Characteristics in Hunan Province Based on Wavelet Transform
Based on the monitoring data of PM2.5 and other five atmospheric pollutants and meteorological data in Hunan Province from 2017 to 2021,the spatial and temporal distribution characteristics of PM2.5 concentration were analyzed.The continuous wavelet transform and wavelet coherence spectrum were used to study the PM2.5 concentration cycle and the corre-lation between PM2.5 and other atmospheric pollutants and meteorological factors.The main influencing factors of PM2.5 concentration were determined.The results showed that the annual average PM2.5 concentration in Hunan Province showed a downward trend,with an average annual decline rate of 4.88%.The monthly average PM2.5 concentration showed a"U"type distribution.The highest concentration was in January 2017(91.9 μg/m3),and the lowest concentration was in June 2020(15.8 μg/m3).The spatial distribution of the annual average of PM2.5 concentration shows the characteristics of high from northeast to southwest,low from northwest to southeast,and the seasonal average of PM2.5 concentration shows the characteris-tics of winter>autumn>spring>summer.There are significant periodic changes in PM2.5 concentration in 14 cities(states),mainly including a long period of about 272 days and a short period of about 36 days.The correlation between PM2.5 concentra-tion and other air pollutants is different at different time-frequency scales.There is a significant positive correlation between PM2.5 concentration and PM10 concentration at all time-frequency scales.On the hourly scale(0~64 d),PM2.5 concentration was positively correlated with O3,CO,NO2 and SO2 concentrations.On the medium time-frequency scale(64~256 d),the correla-tion between PM2.5 concentration and O3 concentration is not obvious,and there is a positive correlation with CO,NO2 and SO2 concentration.On the large time-frequency scale(256~512 d),PM2.5 concentration was negatively correlated with O3 concentration,and positively correlated with NO2 and SO2 concentration.PM2.5 concentration was positively correlated with CO concentration in Changsha and Hengyang,and negatively correlated in Huaihua.The correlation between PM2.5 concentra-tion and meteorological factors is also different at different time-frequency scales.On the hourly frequency scale,PM2.5 is negatively correlated with precipitation,relative humidity and air pressure,positively correlated with temperature and sunshine hours,and positively correlated with wind speed.On the medium-time-frequency scale,the correlation between PM2.5 and various meteorological factors is not obvious;on the large time-frequency scale,PM2.5 is negatively correlated with precipita-tion,temperature and sunshine hours,PM2.5 is positively correlated with air pressure,and the correlation between PM2.5 and rel-ative humidity and wind speed is not obvious.

PM2.5 concentrationpollution characteristicswavelet transforminfluence factorHunan Province

徐赞超、穆述鑫、耿星莉、刘迎云

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南华大学资源环境与安全工程学院,湖南 衡阳 421001

中核建核电建设环保安全与节能技术重点实验室,湖南 衡阳 421001

PM2.5浓度 污染特征 小波变换 影响因素 湖南省

湖南省教育厅科学研究重点项目

17A180

2024

环境科学与技术
湖北省环境科学研究院

环境科学与技术

CSTPCD北大核心
影响因子:0.943
ISSN:1003-6504
年,卷(期):2024.47(3)