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长春大气细颗粒物中多环芳烃的季节变化及健康风险评价

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为研究长春大气细颗粒物(PM2.5)中多环芳烃(PAHs)的季节变化及健康风险评价,于2020年9月至2021年4月采集大气PM2.5样品,测定PM2.5中16种优先控制PAHs的浓度.结果表明,除二苯并(a,h)蒽外,其他15种PAHs均有检出,总质量浓度在0~198.00 ng/m3,平均值为67.80 ng/m3,呈冬季(平均值71.90 ng/m3)>春季(平均值70.50 ng/m3)>秋季(平均值55.20 ng/m3)的特征,PAHs的苯并(a)芘毒性当量季节变化明显,冬季(平均值4.40 ng/m3)显著高于秋季(平均值1.26 ng/m3)和春季(平均值0.38 ng/m3).成人和儿童在冬季的平均终生致癌风险(ILCR)值分别为2.15 × 10-5、2.43 × 10-5,显著高于秋季(成人6.18×10-6、儿童6.98×10-6)和春季(成人1.84×10-6、儿童2.08×10-6),冬季大气PM2.5中PAHs可能对人体存在一定致癌风险.
Seasonal variation and health risk assessment of polycyclic aromatic hydrocarbons in atmospheric fine particulate matter in Changchun
To study the seasonal variation and health risk assessment of polycyclic aromatic hydrocarbons(PAHs)in atmospheric fine particulate matter(PM2.5)in Changchun,atmospheric PM2.5 samples were collected from September 2020 to April 2021.The concentration of 16 priority PAHs in PM2.5 was determined.The results showed that all of the PAHs were detected except DahA.The total mass concentration of 15 PAHs ranged from 0 to 198.00 ng/m3 with an average value of 67.80 ng/m3,presented the tendency of winter(average 71.90 ng/m3)>spring(average 70.50 ng/m3)>autumn(average 55.20 ng/m3).The seasonal variation of BAP toxic equivalents of PAHs was obvious,with winter(average 4.40 ng/m3)was significantly higher than autumn(average 1.26 ng/m3)and spring(average 0.38 ng/m3).The average ILCR values for adults and children in winter were 2.15 × 10-5 and 2.43 × 10-5,respectively,significantly higher than those in autumn(adults 6.18×10-6 and children 6.98×10-6)and spring(adults 1.84×10-6 and children 2.08×10-6),indicating that PAHs in atmospheric PM2.5 in winter might pose a certain carcinogenic risk to human body.

atmospheric particulate matterpolycyclic aromatic hydrocarbonsseasonal variationhealth risk assessment

赵东洋、安淼、刘宝林、于泳

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辽宁工程技术大学环境科学与工程学院,辽宁 阜新 123000

中国科学院湿地生态与环境重点实验室,中国科学院东北地理与农业生态研究所,吉林 长春 130102

长春师范大学化学学院,吉林 长春 130032

大气颗粒物 多环芳烃 季节变化 健康风险评价

长春师范大学自然科学基金资助项目

长师大自科合字[2019]第009号

2024

环境污染与防治
浙江省环境保护科学设计研究院

环境污染与防治

CSTPCD北大核心
影响因子:0.79
ISSN:1001-3865
年,卷(期):2024.46(2)
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