环境污染与防治2024,Vol.46Issue(3) :304-310.DOI:10.15985/j.cnki.1001-3865.2024.03.002

聚醚砜载镧吸附剂的制备及其吸附除磷性能研究

Study on preparation of lanthanum-loaded polyethersulfone adsorbent and its performance on phosphorus removal by adsorption

何东恺 周小国 唐诗琴 朱华 孙凌凯 罗坤 毛旭辉
环境污染与防治2024,Vol.46Issue(3) :304-310.DOI:10.15985/j.cnki.1001-3865.2024.03.002

聚醚砜载镧吸附剂的制备及其吸附除磷性能研究

Study on preparation of lanthanum-loaded polyethersulfone adsorbent and its performance on phosphorus removal by adsorption

何东恺 1周小国 2唐诗琴 1朱华 1孙凌凯 3罗坤 3毛旭辉1
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作者信息

  • 1. 武汉大学资源与环境科学学院,湖北 武汉 430079
  • 2. 长江生态环保集团有限公司,湖北 武汉 430077
  • 3. 长江勘测规划设计研究有限责任公司,湖北 武汉 430010
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摘要

用孔径为3.0μm的聚醚砜(PES)高分子膜材料在质量分数15%的NaOH、摩尔浓度1.42 mol/L的LaCl3最优条件下制备得到了一种PES载镧吸附剂,镧负载质量比达到34.4%,吸附平衡时的磷吸附量最高可达65.1 mg/g,在较宽的pH范围(3.5~6.5)内保持较好的除磷性能,且几乎不受常见的竞争阴离子干扰,具有较强的选择吸附性.PES载镧吸附剂有一定的循环再生能力,在5次吸附/再生循环后,吸附量保持率仍有76.0%,而且动态除磷实验时也能高效除磷,并可再生循环,展示了良好的工程应用前景.

Abstract

Polymeric membrane material polyethersulfone(PES)with pore size of 3.0 μm was used to prepare lanthanum-loaded PES adsorbent under the optimum conditions of 15%mass percentage NaOH and 1.42 mol/L LaCl3,the lanthanum load mass ratio reached 34.4%and its phosphorus equilibrium adsorption capacity reached as high as 65.1 mg/g.It maintained good phosphorus removal performance in a wide range of pH(3.5-6.5),and its adsorption capacity was not affected by the common competing anions,which showed strong adsorption selectivity.Lanthanum-loaded PES adsorbent had good recycling ability.76.0%of the initial phosphorus adsorption capacity could still be maintained after 5 batches of adsorption-regeneration cycles.The dynamic experiment also showed high removal efficiency of phosphorus and good regeneration,which showed a good prospect of engineering application.

关键词

除磷/吸附/载镧/高分子膜材料/聚醚砜

Key words

phosphorus removal/adsorption/lanthanum-loaded/polymeric membrane material/polyethersulfone

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基金项目

国家自然科学基金(52170169)

国家重点研发计划(2019YFD1101300)

中国长江三峡集团有限公司科技项目(202103361)

中国长江三峡集团有限公司科技项目(202103363)

中国长江三峡集团有限公司科技项目(HB/ZB2021130)

出版年

2024
环境污染与防治
浙江省环境保护科学设计研究院

环境污染与防治

CSTPCD北大核心
影响因子:0.79
ISSN:1001-3865
参考文献量23
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