首页|绿狐尾藻基混合填料对生物滤池的脱氮性能及温室气体排放影响

绿狐尾藻基混合填料对生物滤池的脱氮性能及温室气体排放影响

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针对反硝化生物滤池系统处理低碳污水脱氮效率不高及伴随温室气体排放的问题,以收割得到的绿狐尾藻(Myrio-phyllum aquaticum)及其制备的生物炭这两种碳源材料作为滤池填料,构建微型反硝化生物滤池。在投加不同比例的上述两种碳源材料后,连续通入模拟低碳污水,研究滤池的脱氮性能及温室气体排放规律。85 d运行期内,对出水水质及温室气体排放的监测结果显示:绿狐尾藻分解释放有机碳的能力远高于生物炭,以绿狐尾藻为单一填料的滤池脱氮效果最佳,对硝酸盐氮的平均去除率为93。9%,且在试验0~60 d,硝酸盐氮去除率接近100%,总氮平均去除率为76。4%;以生物炭为单一填料的滤池,只在试验0~10 d对硝酸盐氮和总氮有一定去除效果,后续无去除能力;绿狐尾藻与其生物炭按不同比例混合作填料时,整个试验期内对硝酸盐氮平均去除率均高于80%。相比以绿狐尾藻为单一填料,当绿狐尾藻与生物炭质量比为1︰1时,其N2O、CO2和CH4平均排放通量均明显降低,分别降至401。9 μg/(m2·h)、197。8mg/(m2·h)、113。5 mg/(m2·h)。绿狐尾藻可作为反硝化生物滤池处理低碳污水时的外加碳源,与其生物炭混合虽未能进一步提升滤池的脱氮性能,但可进一步减少温室气体的排放。
Impacts of the Myriophyllum aquaticum based mixed filler on denitrification performance and greenhouse gas emissions in biofilters
This study aimed to address the low denitrification efficiency and associated greenhouse gas emissions in the use of biofilter systems for treating low carbon wastewater.By using the residues of Myriophyllum aquaticum and its biochar prepared from it as filter materials,small-scale denitrification biofilters were constructed.Different proportions of the two carbon sources were added,and simulated low carbon wastewater was continuously introduced to investigate the denitrification performance and greenhouse gas emission patterns of the denitrification biofilter.Monitoring results of the 85-day operation period showed that the ability of Myriophyllum aquaticum to decompose and release organic carbon was much higher than that of biochar.When Myriophyllum aquaticum was used as the sole filter material,the denitrification effect was optimal,with an average removal efficiency of 93.9%for nitrate nitrogen.The removal efficiency of nitrate nitrogen remained close to 100%for the first 60 days of the experiment,withan average total nitrogen removal efficiency of 76.4%.In contrast,when biochar was used as the sole filter material,there was only an initial removal effect for nitrate nitrogen and total nitrogen in the first 10 days,with little subsequent removal capability.When Myriophyllum aquaticum and its biochar were mixed in different proportions as filter materials,the average removal efficiency of nitrate nitrogen was above 80%throughout the entire experimental period.Compared with the condition that Myriophyllum aquaticum was used as the sole filter material,when the mass ratio of Myriophyllum aquaticum to biochar was 1︰1,the average emission fluxes of N2O,CH4 and CO2 decreased to 401.9 μg/(m2·h),197.8 mg/(m2·h)and 113.5 mg/(m2·h),respectively.The results of the study indicated that Myriophyllum aquaticum could serve as an external carbon source for treating low carbon wastewater in biofilter systems.When mixed with biochar,though it did not further enhance the denitrification performance of the denitrification biofilters,it did help reduce the greenhouse gas emissions.

Myriophyllum aquaticumbiochardenitrification biofilternitrogen removalgreenhouse gas

陈恒、黄敏、刘锋、李红芳、王彪懿

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武汉理工大学资源与环境工程学院,湖北 武汉 430070

中国科学院亚热带农业生态研究所,亚热带农业生态过程重点实验室,湖南 长沙 410125

绿狐尾藻 生物炭 反硝化生物滤池 脱氮 温室气体

广西重点研发计划项目长沙市自然科学基金青年科学基金项目

AB21220006kq2202321

2024

环境污染与防治
浙江省环境保护科学设计研究院

环境污染与防治

CSTPCD北大核心
影响因子:0.79
ISSN:1001-3865
年,卷(期):2024.46(9)