首页|S/N对硫自养反硝化耦合厌氧氨氧化反应氮素转化的影响

S/N对硫自养反硝化耦合厌氧氨氧化反应氮素转化的影响

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S0基硫自养反硝化耦合厌氧氨氧化(sulfur autotrophic denitrification anammox,S0ADN-Anammox)工艺中普遍存在S/N较高问题,从而造成S0的浪费.为此,通过批次实验,在不考虑S0流失条件下,优化了以S0为电子供体的系统中适宜的S/N,并通过底物控制策略,模拟S0ADN前半程完全反应,仅存在后半程与Anammox的系统环境,讨论在不同S0存在的情况下S0ADN后半程和Anammox对NO2--N的竞争能力.结果表明,在不同的S0投加量条件下,S0ADN-Anammox系统会表现出不同的脱氮性能,当S/N=1,S0ADN-Anammox系统总氮去除率较高,达89%,其中NH4+-N和NO3--N的去除率分别为77%和100%;当只存在NO2--N和NH4+-N时,S0质量浓度越高,Anammox可获得的NO2--N越少,S0ADN后半程对NO2--N的竞争能力要强于Anammox,过高的S/N会影响NH4+-N去除效果.
Effect of S/N on nitrogen transformation in sulfur autotrophic denitrification coupled anaerobic ammonium oxidation reaction
There is a common problem of high S/N in the S0-based sulfur autotrophic denitrification coupled anaerobic ammonium oxidation(sulfur autotrophic denitrification anammox,S0ADN-Anammox)process,resulting in the waste of S0.Thus,batch experiments were conducted to optimize the appropriate S/N in the sulfur autotrophic denitrification coupled anaerobic ammonium oxidation system when S0 was taken as the electron donor without considering the loss of S0.And the first half stage of the complete reaction of S0ADN was simulated through the substrate control strategy,then in the system environment of the second half stage of S0ADN and Anammox,their competitive ability for NO2--N in the presence of different S0 was discussed.The results showed that the S0ADN-Anammox system had a different denitrification performance at different S0 dosage.When S/N=l,the total nitrogen removal rate of the S0ADN-Anammox system was high and reached 89%,of which the removal rates of NH4+-N and NO3--N were 77%and 100%,respectively;when only NO2--N and NH4+-N existed,the higher the S0 mass concentration,the less NO2--N available to Anammox,and the competitive ability for NO2--N in the second half of S0ADN was stronger than Anammox,and too high S/N could affect the NH4+-N removal effect.

S0ADN-Anammoxthe impact of S/Nsubstrate competition relationship

李寓哲、顾晓丹、黄勇

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苏州科技大学环境科学与工程学院,苏州 215009

苏州科技大学环境生物研究所,苏州 215009

硫自养反硝化耦合厌氧氨氧化 S/N的影响 底物竞争关系

国家自然科学基金重点资助项目

51938010

2024

环境工程学报
中国科学院生态环境研究中心

环境工程学报

CSTPCD北大核心
影响因子:0.804
ISSN:1673-9108
年,卷(期):2024.18(7)