激光技术2024,Vol.48Issue(6) :867-875.DOI:10.7510/jgjs.issn.1001-3806.2024.06.012

局域表面等离激元增强的MoS2光电探测器研究

Localized surface plasmon resonance enhanced MoS2 photodetector

程佳宝 唐大秀 谢颖 顾辰杰 刘自军 芦鹏飞 沈祥
激光技术2024,Vol.48Issue(6) :867-875.DOI:10.7510/jgjs.issn.1001-3806.2024.06.012

局域表面等离激元增强的MoS2光电探测器研究

Localized surface plasmon resonance enhanced MoS2 photodetector

程佳宝 1唐大秀 1谢颖 1顾辰杰 1刘自军 1芦鹏飞 2沈祥1
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作者信息

  • 1. 宁波大学高等技术研究院,宁波 315211,中国
  • 2. 北京邮电大学信息光子学与光通信全国重点实验室,北京 100876,中国
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摘要

为了提升2维MoS2光电探测器的响应度、响应速度和响应光谱范围,利用电化学工作站向MoS2块体中插入四庚基阳离子,采用超声辅助剥离工艺获得了高质量的多层MoS2纳米片,并通过旋涂方法制备MoS2光电探测器,在MoS2纳米片上修饰具有双重等离激元共振模式的金纳米棒(Au NRs)来增强入射光与光吸收层的相互作用,提升其光电探测性能与宽光谱响应能力.结果表明,MoS2/Au NRs光电探测器的响应度从2.4×10-3 A/W提高到0.484 A/W,响应时间从50 ms提升到20 ms.上述工作对于简化光电探测器的制备流程,优化新型光电探测器的结构,扩展探测器的可探测光谱范围具有重要意义.

Abstract

In order to enhance the responsivity,response speed and response spectral range of 2-D MoS2 photodetectors,high-quality multilayer MoS2 nanosheets were prepared by inserting tetrahexyl ammonium chloride(THA+)into bulks MoS2 through an electrochemical workstation and ultrasound-assisted exfoliation process.Thereafter,the MoS2 photodetectors were prepared by the spin-coating the prepared MoS2 nanosheets on the substate.Subsequently,the detector was modified by the Au nanorods(Au NRs)with double plasmon modes to further enhance the interaction between the photo sensing layer and the incident light.Experimental results show that the responsivity of the MoS2/Au NRs photodetector is improved from 2.4 × 10-3A/W to 0.484 A/W,and the response time is boosted from 50 ms to 20 ms.In summary,this work not only provides a facile and effective method to expandthe detectable spectral range of the photo detector,but also improve the performance of the photo detector.

关键词

探测器/2维材料/电化学剥离/金纳米棒/局域表面等离激元

Key words

detectors/2-D materials/electrochemical exfoliation/Au nanorods/localized surface plasmon resonance

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出版年

2024
激光技术
西南技术物理研究所

激光技术

CSTPCD北大核心
影响因子:0.786
ISSN:1001-3806
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