首页|二异丙基萘基质3H和14C液闪标准源的稳定性与淬灭校正准确性研究

二异丙基萘基质3H和14C液闪标准源的稳定性与淬灭校正准确性研究

Stability and Quenching Correction Accuracy Study of 3H&14C Liquid Scintillation Reference Sources Based on Diisopropylnaphthalene

扫码查看
为了建立商用液闪液分析水溶液样品中3H、14C 的淬灭校正方法,基于二异丙基萘(Diisopropylnaphthalene,DIN)液闪液制备了3H无淬灭液闪标准源、3H淬灭系列液闪标准源、14C无淬灭液闪标准源和14C淬灭系列液闪标准源.考察了室温、避光条件下标准源的稳定性,16 个月后淬灭系列标准源的校正效率的变化小于0.5%,无淬灭3H、14C标准源的活度值和tSIE值在30 个月的监测中斜率统计值均小于临界值,未观察到不稳定性.比较了DIN体系淬灭系列标准源与甲苯体系淬灭系列标准源对商用液闪液测量核素的校正准确性,结果表明DIN 基质的淬灭系列标准源更适用于目前广泛使用的商用闪烁液(Ultima GoldTM AB、Ultima GoldTM LLT、Optiphase HiSafe 3)测试样品的淬灭校正.
To establish a quenching correction method for 3H and 14C in aqueous samples with commercial liquid scintillation cocktails,unquenched reference sources and quenched series reference sources of 3H and 14C were prepared with DIN(Diisopropylnaphthalene)scintillation cocktails.The stability of the reference sources was investigated in dark condition at room temperature.The change of the correction efficiency of the quenched series of reference sources was less than 0.5%after 16 months.The slopes of activity and tSIE of the unquenching reference sources of 3H and 14C were lower than the critical value during 30 months,which meant that these reference sources were stable.The quenching correction accuracy of toluene and DIN quenched series reference sources was compared by correcting 3H and 14C samples consisted of different commercial liquid scintillation cocktails.As a result,the correction curve of DIN reference sources was more suitable for commercial liquid scintillation cocktails such as Ultima GoldTM AB,Ultima GoldTM LLT and Optiphase HiSafe 3.

ionizing radiation measurementDiisopropylnaphthaleneliquid scintillationquenching3H14Cstability

肖扬、张辉、马彦、刘玫玲、刘皓然、梁珺成、张津肇、赵清、范梓浩、张晗、刘鹏、范富有、戴雄新

展开 >

中国计量科学研究院,北京 100029

中国辐射防护研究院,山西 太原 030006

核药研发转化与精准防护山西省重点实验室,山西 太原 030006

哈尔滨工程大学 烟台研究院,山东 烟台 264000

展开 >

电离辐射计量 二异丙基萘 液闪 淬灭 3H 14C 稳定性

2024

计量学报
中国计量测试学会

计量学报

CSTPCD北大核心
影响因子:0.303
ISSN:1000-1158
年,卷(期):2024.45(11)