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某饮用水源地水体重金属分布特征及健康风险评价

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为探讨湖库型饮用水源地水体重金属的分布特征及引起的人体健康风险,以云南中部某水库饮用水源地水体为研究对象,基于当地生态环境监测部门 2019-2021 年水质监测数据,分析了研究区库区和入库河流水体中 8 种重金属Zn、Pb、Fe、Cd、Mn、Cr6+、As、Hg的质量浓度和分布特征,并运用美国环境保护署(US EPA)推荐的健康风险评价模型进行人体健康风险评价.结果表明:2019-2021 年研究区库区和入库河流水体中均未检出Hg、Cr6+、Pb和Cd,但Zn、As、Fe和Mn均有不同程度检出,且检出质量浓度高值集中在入库河流,入库河流水体重金属质量浓度高值出现在丰水期,库区重金属质量浓度高值出现在枯水期,其中Fe、Mn质量浓度最大值超过我国《生活饮用水卫生标准》(GB 5749-2022)和《地表水环境质量标准》(GB 3838-2002)Ⅲ类水标准限值;经饮水途径,非致癌重金属Pb、Hg、Zn、Fe和Mn对成人和儿童的年健康风险均值处于 10-10/a水平,为无风险;致癌重金属As、Cd和Cr6+对成人的最大年健康风险接近国际辐射防护委员会(ICRP)推荐限值,需引起高度重视,而对儿童的最大年健康风险已超过ICRP推荐限值,有致癌风险;致癌重金属Cr6+和As为儿童致癌风险的决定元素,在儿童饮水方面应优先管控.
Distribution Characteristics and Health Risk Assessment of Heavy Metals Content in a Drinking Water Source Area
In order to explore the distribution characteristics and human health risks of heavy metals in water bodies of lake-reservoir type drinking water sources,the drinking water from a reservoir in a prefecture-level city in central Yunnan Province was selected as the re-searchregion.Based on the data of water quality routine monitoring from the local ecological environment monitoring department in the past three years,the concentration levels and distribution characteristics of eight heavy metals(Zn,Pb,Fe,Cd,Mn,Cr6+,As and Hg)in the reservoir area and inlet river were analyzed.The health risk assessment model recommended by the United States Environmental Protection Agency(US EPA)was used for human health risk assessment.The results show that Hg,Cr6+,Pb and Cd are not detected in the reservoir area and the inflow river in the study area from 2019 to 2021.Zn,As,Fe and Mn are detected to varying degrees,and the high concentra-tions are concentrated in the inflow rivers.The high concentration of heavy metals in the inflow river appeared in the wet season,while the reservoir area appeared in the dry season.Among them,the maximum concentration of iron and manganese is exceeded the limit of drinking water and water environmental quality standards of China.Health risk assessment of metals in the study region shows that non-carcinogenic metals Pb,Hg,Zn,Fe and Mn have no risk to adults are children through drinking water.The maximum carcinogenic risk values of carcino-genic metals As,Cd and Cr6+to adults are almost equal to the recommended limit value of the International Commission on Radiological Pro-tection(ICRP),which needs to be given high priority.However,the maximum health risk level for children has exceeded the recommended limit of ICRP,and there is a risk of cancer.For researched metals,Cr6+and As are the determinants of cancer risk in children and should be given priority control in children's drinking water.

heavy metalhuman health risksdrinking water source

刘淑娟、李国文、鲁瑞梅、杨春涛、张薇、祁云宽、李元

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玉溪师范学院 化学生物与环境学院,云南 玉溪 653100

云南农业大学 动物科学技术学院,云南 昆明 650201

云南省生态环境厅驻玉溪市生态环境监测站,云南 玉溪 653100

玉溪市生态环境科学研究所,云南 玉溪 653100

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重金属 人体健康风险 饮用水源地

国家自然科学基金资助项目云南省科技厅地方本科高校(部分)基础研究联合专项云南省科技厅地方本科高校(部分)基础研究联合专项

319602632017FH001-1252017FH001-043

2024

人民黄河
水利部黄河水利委员会

人民黄河

CSTPCD北大核心
影响因子:0.494
ISSN:1000-1379
年,卷(期):2024.46(2)
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