首页|MXene Hybridized Polymer with Enhanced Electromagnetic Energy Harvest for Sensitized Microwave Actuation and Self-Powered Motion Sensing
MXene Hybridized Polymer with Enhanced Electromagnetic Energy Harvest for Sensitized Microwave Actuation and Self-Powered Motion Sensing
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MXene Hybridized Polymer with Enhanced Electromagnetic Energy Harvest for Sensitized Microwave Actuation and Self-Powered Motion Sensing
Polymeric microwave actuators combining tissue-like softness with pro-grammable microwave-responsive deformation hold great promise for mobile intelligent devices and bionic soft robots.However,their application is challenged by restricted elec-tromagnetic sensitivity and intricate sensing coupling.In this study,a sensitized polymeric microwave actuator is fabricated by hybridizing a liquid crystal polymer with Ti3C2Tx(MXene).Compared to the initial counterpart,the hybrid polymer exhibits unique space-charge polarization and interfacial polarization,resulting in significant improvements of 230%in the dielectric loss factor and 830%in the apparent efficiency of electromag-netic energy harvest.The sensitized microwave actuation demonstrates as the shortened response time of nearly 10 s,which is merely 13%of that for the initial shape memory polymer.Moreover,the ultra-low content of MXene(up to 0.15 wt%)benefits for maintaining the actuation potential of the hybrid polymer.An innovative self-powered sensing prototype that combines driving and piezoelectric polymers is developed,which generates real-time electric potential feedback(open-circuit potential of~3 mV)during actuation.The polarization-dominant energy conversion mechanism observed in the MXene-polymer hybrid structure furnishes a new approach for developing efficient electromagnetic dissipative structures and shows potential for advancing polymeric electromagnetic intelligent devices.
Yu-Ze Wang、Yu-Chang Wang、Ting-Ting Liu、Quan-Liang Zhao、Chen-Sha Li、Mao-Sheng Cao
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School of Materials Science and Engineering,Beijing Institute of Technology,Beijing 100081,People's Republic of China
School of Materials Science and Engineering,Peking University,Beijing 100871,People's Republic of China
School of Mechanical and Material Engineering,North China University of Technology,Beijing 100144,People's Republic of China
Key Laboratory of Functional Inorganic Material Chemistry,Ministry of Education of the People's Republic of China,Heilongjiang University,Harbin 150080,People's Republic of China
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Microwave absorption Electromagnetic response Energy harvest Self-sensing Soft actuator