Abstract
Dielectric and energy storage properties of PbO-SrO-Na2O-Nb2O5-SiO2(PSNNS)thin films with anneal-ing temperature from 700 to 850 ℃ were investigated by measuring their capacitance-electric filed curve and hys-teresis loops.The results show that the highest dielectric constant and energy density are 81.2 and 17.0 J·cm-3,respectively,which is obtained in the sample with annealing temperature of 800 ℃.Annealed from 700 to 800 ℃,the dielectric constant and energy storage perfor-mance of PSNNS films are continuously improved.How-ever,with annealing temperature up to 850 ℃,their dielectric constant decreases,which might be related with the removal of interfacial defects as a function of annealing temperature.Defect is one of the causes of space charge phenomenon,resulting in the increase in dielectric con-stant.Moreover,the microstructure analysis by X-ray diffraction(XRD)and transmission electron microscope(TEM)indicates that the change of crystallization phase and interfacial polarization takes responsibility to the results.
基金项目
National Natural Science Foundation of China(51477012)
Beijing Nova Program(xx2016046)