Advance in reversible Zn anodes promoted by 2D materials

Shu-Yuan Lei ¹Jin-Xiu Feng ¹Yu-Chao Chen ¹Dong Zheng ¹Wen-Xian Liu ¹Wen-Hui Shi ²Fang-Fang Wu ¹Xie-Hong Cao¹

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作者信息

1. School of Materials Science and Engineering,Zhejiang University of Technology,Hangzhou 310014,China
2. Center for Membrane Separation and Water Science and Technology,College of Chemical Engineering,Zhejiang University of Technology,Hangzhou 310014,China
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Abstract

With the growing energy demand associated with high safety and low-cost requirement,aqueous zinc-ion batteries(AZIBs)have been considered as one of the most promising next-generation batteries.However,some key issues,such as uncontrollable dendrites growth,severe cor-rosion,hydrogen evolution and side reactions of Zn anodes during charge/discharge process,have hindered its prag-matic applications.Two-dimensional(2D)materials hold advantages of unique physical and chemical properties,large surface areas and abundant active sites,which have been successfully used to overcome the above shortcomings of Zn anodes in recent years.In this review,the issues and chal-lenges of Zn anodes are outlined.Then,the state-of-the-art progress on Zn anodes modification based on 2D materials such as graphene,2D metal carbides and nitrides(MXenes),2D metal-organic frameworks(MOFs),2D covalent organic frameworks(COFs),2D transition metal compounds and other 2D materials is discussed in detail.Finally,the per-spectives of employing 2D materials in highly reversible Zn anodes are summarized and discussed.

Key words

2D materials/Aqueous zinc-ion battery/Zn anodes/Dendrites growth

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基金项目

Fundamental Research Funds for the Provincial Universities of Zhejiang(RF-B-2020004)

Leading Innovative and Entrepreneur Team Introduction Program of Zhejiang(2020R01002)

National Key Research and Development Project of China(2022YFE0113800)

National Natural Science Foundation of China(51972286)

National Natural Science Foundation of China(21905246)

National Natural Science Foundation of China(22005268)

Natural Science Foundation of Zhejiang Province(LR19E020003)

Natural Science Foundation of Zhejiang Province(LZ21E020003)

Natural Science Foundation of Zhejiang Province(LQ21E020004)

Natural Science Foundation of Zhejiang Province(LQ20B010011)

出版年

2024

稀有金属(英文版)

中国有色金属学会

稀有金属(英文版)

CSTPCDEI

影响因子：0.801

ISSN：1001-0521

参考文献量130

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