Solar-driven photothermal catalytic CO2 conversion:a review

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外文摘要：It is highly desirable to seek green and sus-tainable technologies,such as employing photothermal effects to drive energy catalysis processes to address the high energy demand and associated environmental impacts induced by the current methods.The photothermocatalysis process is an emerging research area with great potential in efficiently converting solar energy through various cat-alytic reactions.However,achieving simultaneously high conversion efficiency,cyclability,and durability is still a daunting challenge.Thus,tremendous work is still needed to enhance solar photothermal catalytic conversion and promote its large-scale applications.This review developed the principles of coupling solar photon and thermal fields underlying the photothermal effect,exploration of efficient nanocatalysts,development of optofluidic reactor model,and photothermal synergistic-driven CO2 reduction mech-anisms.The ultimate goal was to provide an effective approach that can effectively convert solar energy into photocarriers/hot-electrons and heat,and importantly,can couple them to regulate catalysis reaction pathways toward the production of value-added fuel and chemical energy.

外文关键词：

PhotochemistryPhotothermalCO2 catalytic conversionNanomaterialSolar fuels and chemicals

作者：

Bachirou Guene Lougou、Bo-Xi Geng、Ru-Ming Pan、Wei Wang、Tian-Tian Yan、Fang-Hua Li、Hao Zhang、Oraléou Sangué Djandja、Yong Shuai、Meisam Tabatabaei、Daniel Sabi Takou

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作者单位：

School of Energy Science and Engineering,Harbin Institute of Technology,Harbin 150001,China

MIIT Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage,Harbin Institute of Technology,Harbin 150001,China

State Key Laboratory of Urban Water Resource and Environment,Harbin Institute of Technology,Harbin 150090,China

School of Electrical Engineering and Automation,Harbin Institute of Technology,Harbin 150001,China

Guangdong Provincial Key Laboratory of Distributed Energy Systems,Engineering Research Center of None-Food Biomass Efficient Pyrolysis and Utilization Technology of Guangdong Higher Education Institutes,Dongguan University of Technology,Dongguan 523808,China

Higher Institution Centre of Excellence(HICoE),Institute of Tropical Aquaculture and Fisheries(AKUATROP),Universiti Malaysia Terengganu,21030 Kuala Nerus,Malaysia

Department of Biomaterials,Saveetha Dental College,Saveetha Institute of Medical and Technical Sciences,Chennai 600 077,India

École Polytechnique d'Abomey-Calavi,University of Abomey-Calavi,2009 Cotonou,Benin

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基金：

China National Key Research and Development Plan ProjectNational Natural Science Foundation of China

项目编号：

2018YFA070230052227813

出版年：

2024

DOI：

10.1007/s12598-024-02638-4

稀有金属(英文版)