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中国近海及西北太平洋气溶胶铁的研究进展

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总结中国近20年来近海及西北太平洋区域海洋气溶胶中铁的研究进展。从铁排放清单的角度,介绍从沙尘铁清单到人为源铁清单建立的历程,包括总铁和可溶性铁;总结气溶胶中铁浓度的测量方法和来源解析技术的最新进展,强调未来海洋总铁和可溶铁在线测量的重要性,在线测量是获得高分辨率海洋气溶胶铁时空分布特征的关键;此外,指出新兴的铁同位素分析技术可实现对气溶胶铁来源的定量解析,同时将铁的在线测量技术与源解析受体模型结合是定量认识铁来源的新路径;最后总结气溶胶铁沉降对海洋生态和气候的影响,气溶胶铁沉降对浮游植物的生长具有明显的促进作用,但铁沉降气候效应的定量评估仍存在较大的不确定性。未来应加强对海洋大气铁观测数据的积累,深入对铁化学相关机制的研究,并及时推动大气与海洋模型的结合。
Atmospheric iron in Chinese marginal seas and the Northwest Pacific:A review
The research progress of iron in marine aerosol in Chinese marginal seas and the Northwest Pacific Ocean in recent 20 years was reviewed.First,the development history of iron emission inventory,from natural dust source to anthropogenic sources was introduced,including both total Fe and soluble Fe.Second,the latest progress of the measurement methods and source apportionment techniques for Fe in marine aerosol was discussed,with an emphasis on the importance of online measurement of total Fe and soluble Fe,which was the key for obtaining the high spatiotemporal distribution of Fe in marine aerosol.In addition,this study pointed out that the new emerging iron isotope analysis technique could be used for quantitative apportionment of iron sources,and the combination of online measurements with receptor models of source apportionment was a new way to provide quantitative understanding of iron sources.Finally,the impacts of iron deposition on marine ecology and climate were summarized.Studies had revealed that atmospheric iron deposition could significantly stimulate phytoplankton growth,but large uncertainties remained regarding its climate effects quantification.Future research was needed on marine aerosol Fe measurement data accumulation,in-depth analysis of related mechanisms of iron chemistry,and the integration between atmospheric and oceanic models.

marine aerosolironemission inventorysource apportionmentocean response

张天乐、郑玫

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北京大学环境科学与工程学院,北京 100871

海洋气溶胶 排放清单 来源解析 海洋响应

国家自然科学基金

42030708

2024

中国环境科学
中国环境科学学会

中国环境科学

CSTPCDCHSSCD北大核心
影响因子:2.174
ISSN:1000-6923
年,卷(期):2024.44(2)
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