中国环境科学2024,Vol.44Issue(3) :1212-1224.

秸秆燃烧气溶胶的气象反馈及其棕碳吸光效应

Meteorological feedback and brown carbon absorption effect of straw burning aerosols

王璐瑶 张磊 安兴琴 王格慧
中国环境科学2024,Vol.44Issue(3) :1212-1224.

秸秆燃烧气溶胶的气象反馈及其棕碳吸光效应

Meteorological feedback and brown carbon absorption effect of straw burning aerosols

王璐瑶 1张磊 2安兴琴 1王格慧3
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作者信息

  • 1. 中国气象科学研究院灾害天气国家重点实验室,北京 100081;中国气象科学研究院气象影响与风险研究中心,北京 100081
  • 2. 中国气象科学研究院灾害天气国家重点实验室,北京 100081;中国气象局大气化学重点开放实验室,北京 100081
  • 3. 华东师范大学地理科学学院,上海 200062
  • 折叠

摘要

本文利用WRF-Chem模式模拟研究了2013年6月华北地区秸秆燃烧排放气溶胶的气象效应,并对秸秆燃烧产生的吸收性有机气溶胶(即棕碳或BrC)的光吸收效应进行分析.设置4组敏感性试验,通过与AERONET观测结果对比分析了BrC对光吸收的影响.结果表明:模式较好再现了研究时段内各变量变化;在不考虑BrC吸收的情况下,秸秆燃烧产生的气溶胶在主要的农业产区造成地表短波辐射的减弱,月平均值减弱约 12.42W/m2,且造成近地面降温而2km以上高空增温,其中近地面温度降幅为0.12~3.64℃,致使边界层趋于稳定,垂直扩散能力减弱;气压整体升高,正变压中心与火点密集区域重合.同时,秸秆燃烧引发近地面较强的风辐散,抑制海洋高湿气团向秸秆燃烧区域的水平输送.在考虑BrC的吸收作用后,光学参数的模拟效果得到了一定提升,AAOD 模拟值与观测值的拟合线性斜率由 0.47 升至 0.53,AOD 斜率值由 0.19 升至 0.21.生物质燃烧排放 BrC 对气溶胶消光的影响显著,如AAOD与AOD均出现不同程度的上升.

Abstract

Straw burning is a major source of biomass combustion in North China,significantly impacting air quality.Using the WRF-Chem model,we simulated the meteorological effects of aerosol emissions from straw burning in June 2013 and conducted a preliminary analysis of the light-absorbing properties of brown carbon(BrC)produced during straw burning.We conducted four sensitivity experiments,comparing the impact of BrC on light absorption with AERONET observations.Results showed that the model effectively captured variations in various parameters during the study period.Without considering BrC absorption,straw burning led to a reduction in surface shortwave radiation,causing a monthly average decrease of approximately 12.42 W·m-2 in major agricultural regions.This resulted in near-surface cooling,warming above 2km,and reduced vertical diffusion,stabilizing the boundary layer.There was an overall increase in atmospheric pressure,coinciding with fire hotspot areas.Straw burning also induced strong near-surface wind divergence,hindering the horizontal transport of moist air masses from the ocean.Considering BrC absorption,the simulation of optical parameters significantly improved.The linear fit slope between simulated Absorption Aerosol Optical Depth(AAOD)and observed values increased from 0.47 to 0.53,and the slope of Aerosol Optical Depth(AOD)increased from 0.19 to 0.21.Biomass burning emissions of BrC had a notable impact on aerosol extinction,leading to increased AAOD and AOD to varying degrees.

关键词

生物质燃烧/BrC/光吸收/WRF-Chem模式/华北地区

Key words

biomass combustion/BrC/light absorption/WRF-Chem model/North China

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基金项目

国家自然科学基金资助项目(42130704)

国家自然科学基金资助项目(41975173)

国家自然科学基金资助项目(42207134)

出版年

2024
中国环境科学
中国环境科学学会

中国环境科学

CSTPCDCHSSCD北大核心
影响因子:2.174
ISSN:1000-6923
参考文献量58
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