首页|三江平原农田排水期流域水体CH4排放特征及影响因素

三江平原农田排水期流域水体CH4排放特征及影响因素

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在施肥和土壤淋溶等多种因素的影响下,农业流域水体甲烷(CH4)的源汇关系尚不明确,目前对于农业流域水体CH4排放的监测和研究仍然不足.本研究选取三江平原的浓江流域为研究对象,利用顶空平衡法和扩散模型法对该流域不同水体的CH4浓度和排放通量进行监测和估算.结果表明:浓江流域水体普遍为CH4的排放源,鸭绿河、浓江河流、沟渠和稻田水体的CH4排放通量范围分别为0.51~99.60、0.97~20.44、4.13~20.90和24.84~58.07mg/(m2.d),且沟渠和稻田水体的CH4排放通量较高,分别为浓江河流的2倍和7倍.在鸭绿河干流和沟渠水体中,CH4浓度与pH值和溶解氧(DO)均呈显著负相关,浓江干流的CH4浓度与DO呈显著正相关.浓江干流和沟渠水体的CH4浓度与溶解性有机碳(DOC)呈显著正相关,表明排水期农业有机肥的使用会促进水体CH4的产生.流经湿地浅水区和受农田施肥影响的河段水体具有较高的CH4浓度和排放通量,表明CH4排放受到了土地利用方式的显著影响.相比于全球其他农业河流,排水期浓江流域河水在排水期具有较高的CH4浓度和较低的CH4排放通量,较低风速缓解了水-气界面的排放.而沟渠水体排水期间较低的CH4排放通量主要受富氧状态的影响.三江平原作为典型的东北黑土农业区,探究其农业流域CH4的产生和排放对于未来区域的碳收支平衡和碳排放评估具有重要意义.
Characteristics of methane(CH4)emissions and influencing factors in surface waters of farmland during the drainage period in the Sanjiang Plain
Under the influences of fertilization and soil leaching,the source and sink effects of methane(CH4)in surface waters of agricultural watersheds remain unclear.Currently,the monitoring and studying of CH4 emissions in waters of agricultural watersheds are still inadequate.This study focused on the Nongjiang River Basin within the Sanjiang Plain,employing the headspace equilibrium method and the diffusion model approach to precisely monitor and estimate the CH4 concentrations and fluxes in various water bodies of the basin.The results showed that the water bodies in the Nongjiang watershed generally acted as sources of atmospheric CH4.The CH4 fluxes at the water-air interfaces of the Yalü River,Nongjiang River,ditches,and paddy fields ranged from 0.51 to 99.60,0.97 to 20.44,4.13 to 20.90,and 24.84 to 58.07mg/(m2·d),respectively.The CH4 fluxes from ditches and paddy fields were 2 and 7 times higher than those of the Nongjiang River,respectively.In the Yalü River and ditches,CH4 concentrations correlated significantly and negatively with pH and dissolved oxygen(DO),while the CH4 concentrations in the Nongjiang River correlated significantly and positively with DO.The CH4 concentrations in the Nongjiang River and ditches water bodies were significantly positively correlated with dissolved organic carbon(DOC),indicating that the use of agricultural organic fertilizer during the drainage period promotes the production of CH4.The study found that river reaches that flow through shallow wetlands and agricultural areas generally have higher CH4 concentrations and fluxes,suggesting the effects of land use patterns on CH4 emissions were important.Compared with other agricultural watersheds globally,the Nongjiang River during the drainage period has higher CH4 concentrations and lower CH4 fluxes,low wind speed eased the CH4 diffusion at water-air interface;while the the low CH4 flux in the ditch waters during the drainage period mainly resulted from the high DO.As a typical agricultural area in the northeastern black soil region of China,understanding the production and emission of CH4 in the agricultural watersheds is of great significance for future carbon budget balances and carbon emission assessments in this region.

agricultural watersheddrainage periodgreenhouse gas CH4production and emission

刘凯明、张海、李霞、王明国、杨涛、李军、白莉、刘小龙

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天津师范大学,天津市水资源与水环境重点实验室,天津 300387

天津师范大学,地理与环境科学学院,天津 300387

中国地质调查局,水文地质环境地质调查中心,河北 保定 071051

农业流域 排水期 温室气体CH4 产生与排放

中国地调局地质调查项目中国地调局地质调查项目天津市科技局项目国家自然科学基金国家自然科学基金

DD20190534DD2022175421ZYJDJC000904167235141661144029

2024

中国环境科学
中国环境科学学会

中国环境科学

CSTPCDCHSSCD北大核心
影响因子:2.174
ISSN:1000-6923
年,卷(期):2024.44(6)
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