首页|2014~2020年夏季高温热浪期间臭氧变化特征——以长三角地区典型城市为例

2014~2020年夏季高温热浪期间臭氧变化特征——以长三角地区典型城市为例

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选取上海、南京、杭州作为长三角地区典型代表城市,基于观测资料和WRF-CMAQ模式,分析了 3个城市2014~2020年夏季高温热浪期间臭氧(O3)的变化特征。结果表明:3个城市夏季高温热浪强度均呈现先上升后下降再上升的趋势,2016和2017年为高温热浪超强年,2014和2018年为高温热浪弱年。热浪期间O3逐小时平均浓度变化呈现"单峰单谷"型,在13:00、14:00达到峰值,6:00达到谷值。各个城市热浪期间平均日最大O3浓度、O3昼夜间平均浓度和O3日最大8h滑动平均浓度(MDA8O3)年际变化趋势相似,上海下降趋势明显,南京呈先上升后下降趋势,杭州总体呈下降趋势,且各城市热浪期间O3浓度随温度的阶段变化特征明显。WRF-CMAQ模式可以较好地模拟3个城市热浪期间的MDA8O3,模拟发现气象条件变化和前体物排放变化对各个城市热浪期间MDA8O3变化的影响不同,气象条件变化对上海热浪期间MDA8O3下降起主导作用,南京热浪期间MDA8O3主要受排放变化影响,杭州热浪期间MDA8O3的变化受气象和排放综合作用的共同影响。同时持续的高温并不是影响O3浓度的唯一气象因素,平均海平面气压和风速对热浪期间MDA8O3也有显著的影响。
Characteristics of ozone variations during summer heat waves in typical cities in the Yangtze River Delta Region from 2014 to 2020
Three cities in the Yangtze River Delta(YRD),Shanghai,Nanjing and Hangzhou,were selected as typical representative cities to analyze the characteristics of ozone(O3)variations during the summer heat waves from 2014 to 2020 based on observations and WRF-CMAQ model.The results showed that the intensity of summer heat waves in the three cities showed an increasing,then decreasing,then increasing trend,with 2016 and 2017 being the years of super heat waves and 2014 and 2018 being the years of weak heat waves.The hourly O3 concentrations during the heat waves showed a"single peak,single valley"pattern,peaking at 13:00 or 14:00 and reaching valley values at 6:00.Interannual variations of the average daily maximum O3 concentrations,the average daytime and nighttime O3 concentrations and Maximum Daily 8-Hour Average O3(MDA8O3)during the heat waves were similar in each city,with a significant decreasing trend in Shanghai,an increasing and then decreasing trend in Nanjing,and a decreasing trend in Hangzhou in general,and O3 concentrations during the heat waves were characterized by significant phase changes with temperature in each city.The WRF-CMAQ model could well simulate MDA8O3 during the heat waves in the three cities.Model results showed that the variations in meteorological conditions and precursor emissions have different effects on the changes in MDA8O3 during the heat waves in each city.Variations in meteorological conditions dominated the decrease in MDA8O3 during the heat waves in Shanghai,while variations in MDA8O3 in Nanjing were mainly influenced by variations in emissions,and variations in MDA8O3 in Hangzhou were influenced by the combined effects of meteorology and emissions.Meanwhile,persistent high temperature was not the only meteorological factor affecting O3 concentration,mean sea level pressure and wind speed also had a significant effect on MDA8O3 during the heat waves.

O3high-temperature heat wavesYangtze River DeltaWRF-CMAQ

丁嘉豪、谢晓栋、龚康佳、薛刘铖、胡建林

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南京信息工程大学长望学院,江苏省大气环境监测与污染控制高技术研究重点实验室,江苏南京 210044

南京信息工程大学环境科学与工程学院,大气环境与装备技术协同创新中心,江苏省大气环境监测与污染控制高技术研究重点实验室,江苏南京 210044

臭氧(O3) 高温热浪 长三角地区 WRF-CMAQ

2024

中国环境科学
中国环境科学学会

中国环境科学

CSTPCDCHSSCD北大核心
影响因子:2.174
ISSN:1000-6923
年,卷(期):2024.44(12)