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卫星遥感的山西HCHO柱浓度长期变化趋势

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利用 臭氧检测仪(OMI)HCHO 柱浓度数据及其他t辅助数据,研究了 2013~2022 年 5~8月去除气温影响的山西HCHO柱浓度长期变化趋势,以及天然源 VOCs(BVOCs)和人为源 VOCs(AVOCs)排放的变化在 HCHO柱浓度变化中的作用。结果表明,研究时段山西HCHO柱浓度均值介于4。1×1015~53。6×1015molecule/cm2之间,年均 14。3×1015molecule/cm2,2013~2018年呈上升趋势,2019~2022 年波动下降,HCHO柱浓度乡村普遍高于城市。去除气温影响后,相较于2013~2017 年,2018~2022 年 HCHO 柱浓度下降区多位于人类活动密集的城镇,上升区多分布于受人为活动影响较小的乡村。在HCHO柱浓度受气温显著影响区域中,大同北部HCHO柱浓度上升与农用地的BVOCs排放增加有关;忻州西部-吕梁北部HCHO柱浓度上升与农用地e、稠密灌木、混交林、稀树草原的 BVOCs排放增加有关;晋中中部和临汾南部-运城北部HCHO 柱浓度的下降,是 AVOCs 和 BVOCs排放共同下降的结果,并且 AVOCs 减排有重要作用。
Long-term trends of HCHO columns in Shanxi Province based on satellite remote sensing
The long-term trends of formaldehyde(HCHO)column in Shanxi Province from May to August over the period 2013~2022 were analyzed,using satellite measurements from Ozone Monitoring Instrument(OMI)and auxiliary data.The research examines the influence of biogenic volatile organic compounds(BVOCs)and anthropogenic volatile organic compounds(AVOCs)emissions on the observed variations in HCHO levels.Results indicate that the average HCHO column ranged from 4.1×1015 to 53.6x1015 molecules/cm2,with an annual mean of 14.3 × 1015 molecules/cm2.From 2013 to 2018,HCHO column exhibited an increasing trend,followed by a fluctuating decline from 2019 to 2022.Rural areas consistently showed higher HCHO concentrations compared to urban regions.After removing temperature effects,decreases in HCHO concentrations were observed mostly in urban areas with intense human activities,while increases were observed in rural villages with minimal anthropogenic influence.In temperature-sensitive regions,the rise in HCHO concentrations in northern Datong was attributed to increased BVOCs emissions from croplands.Similarly,in western Xinzhou to northern Lüliang,elevated HCHO concentrations were linked to higher BVOCs emissions from croplands,dense shrublands,mixed forests,and savannas.Conversely,central Jinzhong and southern Linfen to northern Yuncheng experienced reductions in HCHO concentrations due to simultaneous decreases in both AVOCs and BVOCs emissions,with reductions in AVOCs playing a particularly significant role.

HCHO columnsVOCssatellite remote sensingShanxitemperaturelandcover

杨爱琴、于小红、陈玲、闫世明、朱凌云、郭伟、李明明、李雁宇、李莹、贺洁颖

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山西省气象科学研究所,中国气象局温室气体及碳中和监测评估中心山西分中心,山西太原 030002

中国气象局五台山云物理野外科学试验基地,山西太原 030002

中国科学院大学地球与行星学院,北京 100049

中国科学院大气物理研究所,北京 100029

北京师范大学地理科学学部,北京 100875

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甲醛(HCHO)柱浓度 挥发性有机物(VOCs) 卫星遥感 山西 气温 土地覆盖

2024

中国环境科学
中国环境科学学会

中国环境科学

CSTPCDCHSSCD北大核心
影响因子:2.174
ISSN:1000-6923
年,卷(期):2024.44(12)