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城市尺度温室气体排放反演研究进展及发展趋势

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城市是二氧化碳(CO2)和甲烷(CH4)排放的热点区域,占全球人为源总排放量的40%~50%,因此对其排放量的准确量化,直接影响着各国气候变化政策的制定与实施。虽然排放清单方法是当前核算排放量的最主要手段,但大量对比研究表明,温室气体排放量在城市尺度上估算的不确定性依旧大于50%,因此亟需开展城市尺度上温室气体排放量的准确核算,进而降低排放清单的不确定性。而基于浓度观测和大气传输模型的反演方法,从2010年起逐渐被用于城市尺度温室气体排放量的反演研究,但对浓度观测站点选取和排放量反演方法依旧存在认识的不统一与偏差。在我国制定"双碳"政策的战略背景下,本文系统梳理和综述了当前城市尺度温室气体排放量反演的研究进展,重点分析该方法面临的困难和挑战,并指出相较于国外已开展的研究,我国当前城市尺度的温室气体浓度观测网络依旧欠缺,限制了温室气体排放量时空格局和组分的有效拆分。而结合中精度浓度观测网络,并同时发展1km及以下空间分辨率的排放清单和气象驱动场,是未来准确解析城市尺度温室气体排放总量及其时空格局的重要发展方向。通过系统总结当前城市尺度温室气体排放量的研究现状、进展及问题,以及未来潜在发展趋势,预计可为我国"双碳"战略的实施提供方法参考和理论借鉴。
Review of the greenhouse gas emission inversion approaches at city scale and future development trends
Urban areas are hotspots for carbon dioxide(CO2)and methane(CH4),accounting for 40%to 50%of the global anthropogenic emissions.Therefore,the accurate quantification of their emissions directly impacts the formulation and implementation of climate change policies.The emission inventories are currently the main approach to account for emissions.However,numerous studies have shown that the uncertainty of greenhouse gas inventories at the urban scale is still larger than 50%.Hence,there is an urgent need to reduce the uncertainty in emission inventories.Inverse estimation methods,which is based on concentration observations and atmospheric transport model,have gradually been used for the estimation of urban-scale greenhouse gas emissions since 2010.However,there still exists many knowledge gaps for this approach.To meet the goal of"dual carbon"as announced in 2021,this paper reviews the research progress of urban-scale greenhouse gas emissions and discussed recent difficulties and challenges.It points out that the greenhouse gas concentration observation network is still lacking in China.And the use of medium-precision concentration observation networks and simultaneously developing of emission inventories and meteorological fields with spatial resolutions of 1km are important directions to accurately resolve the total emissions and spatiotemporal patterns of greenhouse gases at the urban scale in the future.By systematically summarizing the current research status,progress,and issues related to urban-scale greenhouse gas emissions in this paper,it is expected to provide methodological references and theoretical insights for the implementation of China's"dual carbon"strategy.

greenhouse gasemission inversiontower-based siteatmospheric transport model

胡诚、张俊清、刘慧丽、史雪静、孙帆、肖薇

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南京林业大学生态与环境学院,江苏南京 210018

南京信息工程大学,中国气象局生态系统碳源汇重点开放实验室大气环境中心,江苏南京 210044

温室气体 排放量反演 高塔 大气传输模型

2024

中国环境科学
中国环境科学学会

中国环境科学

CSTPCDCHSSCD北大核心
影响因子:2.174
ISSN:1000-6923
年,卷(期):2024.44(12)