首页|Towards catalytic reactions of Cu single-atom catalysts:Recent progress and future perspective

Towards catalytic reactions of Cu single-atom catalysts:Recent progress and future perspective

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One of the urgent and challenging topics in diversified sustainable energy conversion is the development of high-performance,low-cost,and well durable catalysts.Cu single-atom catalysts(SACs)have become promising catalysts for diversified sustainable energy conversion due to their capability to maximize the utilization efficiency,acquire modulated electronic structure and optimized binding strength with inter-mediates.In this review,we have provided an interview of the recent progress achieved in the field of electrocatalysis,photocatalysis,and heterogeneous reaction based on Cu SACs.Started by this review,we have summarized some advanced synthetic strategies for the construction of Cu SACs.Subsequently,the performance-improving strategies are discussed in terms of the coordination environments of the re-action center,reaction mechanism and selectivity,based on free energy diagram and electron structure analysis.Finally,the remaining issues,challenges,and opportunities of Cu SACs are also provided,afford-ing a perspective for future studies.This review not only offers us a deep understanding on the catalytic mechanism of Cu SACs for energy conversion,but also encourages more endeavors in prompting their practical application.

Cu SACsEnergy conversionCatalysisCoordination environment

Yitao Zhao、Lei Tao

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Jiangsu Province Engineering Research Center of Special Functional Textile Materials,Changzhou Vocational Institute of Textile and Garment,Changzhou 213164,China

Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology,Advanced Catalysis and Green Manufacturing Collaborative Innovation Center,School of Petrochemical Engineering,Changzhou University,Changzhou 213164,China

Postgraduate Research & Practice Innovation Program of Jiangsu ProvinceBasic Science(Natural Science)Research Project of Colleges and Universities of Jiangsu ProvinceChangzhou Sci&Tech Program,ChinaChangzhou Sci&Tech Program,China

KYCX21_279521KJB540001CJ20220180CJ20210042

2024

10.1016/j.cclet.2023.108571

中国化学快报(英文版)
中国化学会

中国化学快报(英文版)

CSTPCD
影响因子：0.771
ISSN：1001-8417
年,卷(期)：2024.35(2)
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