首页|Recent progress and prospects of electrolytes for electrocatalytic nitrogen reduction toward ammonia

Recent progress and prospects of electrolytes for electrocatalytic nitrogen reduction toward ammonia

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Electrochemical nitrogen reduction reaction(ENRR)provides a promising strategy to achieve sustainable synthesis of ammonia.However,despite great efforts devoted to this research field,the problems such as low energy efficiency and weak selectivity still impede its practical implementation.Most of the research to date has been concentrated on creating sophisticated electrocatalysts,and adequate knowledge of elec-trolytes is still lacking.Herein,the recent progress in electrolytes for ENRR,including alkaline,neutral,acidic,water-in-salt,organic,ionic liquid,and mixed water-organic electrolytes,is thoroughly reviewed to obtain an in-depth understanding of their effects on electrocatalytic performance.Recently developed representative electrocatalysts in various types of electrolytes are also introduced,and future research priorities of different electrolytes are proposed to develop new and efficient ENRR systems.

Electrocatalytic nitrogen reductionAmmoniaElectrolytesProduction rateFaradaic efficiency

Sajid Mahmood、Haiyan Wang、Fang Chen、Yijun Zhong、Yong Hu

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Key Laboratory of the Ministry of Education for Advanced Catalysis Materials,Department of Chemistry,Zhejiang Normal University,Jinhua 321004,China

The Center for Applied Mathematics and Bioinformatics(CAMB),Gulf University for Science and Technology,Mishref 32093,Kuwait

Hangzhou Institute of Advanced Studies,Zhejiang Normal University,Hangzhou 311231,China

国家自然科学基金浙江省自然科学基金重大项目浙江省自然科学基金重大项目Zhejiang Provincial Ten Thousand Talent ProgramKey Science and Technology Project of Jinhua City

22272150LD22B030002LZ23B0300022021R510092020-1-044

2024

中国化学快报(英文版)
中国化学会

中国化学快报(英文版)

CSTPCD
影响因子:0.771
ISSN:1001-8417
年,卷(期):2024.35(4)
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