中国化学快报(英文版)2024,Vol.35Issue(5) :57-65.DOI:10.1016/j.cclet.2023.108954

Recent progress of MgO-based materials in CO2 adsorption and conversion:Modification methods,reaction condition,and CO2 hydrogenation

Zixuan Zhu Xianjin Shi Yongfang Rao Yu Huang
中国化学快报(英文版)2024,Vol.35Issue(5) :57-65.DOI:10.1016/j.cclet.2023.108954

Recent progress of MgO-based materials in CO2 adsorption and conversion:Modification methods,reaction condition,and CO2 hydrogenation

Zixuan Zhu 1Xianjin Shi 1Yongfang Rao 2Yu Huang3
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作者信息

  • 1. Key Laboratory of Aerosol Chemistry & Physics,State Key Laboratory of Loess and Quaternary Geology(SKLLQG),Institute of Earth Environment,Chinese Academy of Sciences(CAS),Xi'an 710061,China;Center for Excellence in Quaternary Science and Global Change,Chinese Academy of Sciences,Xi'an 710061,China;University of Chinese Academy of Sciences,Beijing 100049,China
  • 2. Department of Environmental Science and Engineering,Xi'an Jiaotong University,Xi'an 710049,China
  • 3. Key Laboratory of Aerosol Chemistry & Physics,State Key Laboratory of Loess and Quaternary Geology(SKLLQG),Institute of Earth Environment,Chinese Academy of Sciences(CAS),Xi'an 710061,China;Center for Excellence in Quaternary Science and Global Change,Chinese Academy of Sciences,Xi'an 710061,China
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Abstract

Integrated CO2 capture and conversion of(ICCC)is one of the most effective solutions to reduce anthro-pogenic CO2 emissions,which has attracted extensive public attention.Dual functional materials(DFMs),including adsorbent and catalyst,are the key components to achieve ICCC.Magnesium oxide(MgO)is an ideal adsorbent for ICCC,since it is characterized by high theoretical adsorption capacity,low cost,low energy consumption and extensive sources.It can also be used as DFMs in combination with the Ni catalysts.MgO not only can act as an adsorbent in DFMs but also enhance the catalytic performance of Ni.This review summarizes the advantages and modification methods of MgO as adsorbent and the in-fluence of its adsorption conditions on the adsorption performance.Moreover,the important role of MgO in facilitating the catalytic conversion of CO2 is highlighted.Future research focuses are proposed for the development of MgO based DFMs with high adsorption capacity,high stability,conversion,and selectivity as well as low cost and energy consumption.

Key words

CO2/ICCC/MgO/Adsorption/Conversio

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基金项目

中国科学院战略规划重点项目(XDA23010300)

中国科学院战略规划重点项目(XDA23010000)

国家自然科学基金(51878644)

国家自然科学基金(41573138)

Plan for"National Youth Talents"of the Organization Department of the Central Committee()

出版年

2024
中国化学快报(英文版)
中国化学会

中国化学快报(英文版)

CSTPCDCSCD
影响因子:0.771
ISSN:1001-8417
参考文献量146
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