首页|Recent progress of MgO-based materials in CO2 adsorption and conversion:Modification methods,reaction condition,and CO2 hydrogenation
Recent progress of MgO-based materials in CO2 adsorption and conversion:Modification methods,reaction condition,and CO2 hydrogenation
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Integrated CO2 capture and conversion of(ICCC)is one of the most effective solutions to reduce anthro-pogenic CO2 emissions,which has attracted extensive public attention.Dual functional materials(DFMs),including adsorbent and catalyst,are the key components to achieve ICCC.Magnesium oxide(MgO)is an ideal adsorbent for ICCC,since it is characterized by high theoretical adsorption capacity,low cost,low energy consumption and extensive sources.It can also be used as DFMs in combination with the Ni catalysts.MgO not only can act as an adsorbent in DFMs but also enhance the catalytic performance of Ni.This review summarizes the advantages and modification methods of MgO as adsorbent and the in-fluence of its adsorption conditions on the adsorption performance.Moreover,the important role of MgO in facilitating the catalytic conversion of CO2 is highlighted.Future research focuses are proposed for the development of MgO based DFMs with high adsorption capacity,high stability,conversion,and selectivity as well as low cost and energy consumption.
CO2ICCCMgOAdsorptionConversio
Zixuan Zhu、Xianjin Shi、Yongfang Rao、Yu Huang
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Key Laboratory of Aerosol Chemistry & Physics,State Key Laboratory of Loess and Quaternary Geology(SKLLQG),Institute of Earth Environment,Chinese Academy of Sciences(CAS),Xi'an 710061,China
Center for Excellence in Quaternary Science and Global Change,Chinese Academy of Sciences,Xi'an 710061,China
University of Chinese Academy of Sciences,Beijing 100049,China
Department of Environmental Science and Engineering,Xi'an Jiaotong University,Xi'an 710049,China
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中国科学院战略规划重点项目中国科学院战略规划重点项目国家自然科学基金国家自然科学基金Plan for"National Youth Talents"of the Organization Department of the Central Committee