首页|Facile synthesis of high-brightness green-emitting carbon dots with narrow bandwidth towards backlight display

Facile synthesis of high-brightness green-emitting carbon dots with narrow bandwidth towards backlight display

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High-performance carbon dots(CDs)allowing the application in high-end display devices are highly de-sirable and usually limited by the absence of simple and easy synthesis methods.In this work,we ex-ploited an easy-to-implement strategy for the one-step synthesis of green-emitting CDs(G-CDs)with superb optical properties.The G-CDs were synthesized using m-phenylenediamine(m-PD)as a single pre-cursor,and the reaction reacted at 180 ℃ for 12 h The resultant G-CDs exhibit high-purity and excitation-independent green fluorescence with the photoluminescence(PL)peak located at 516 nm,full width at half maximum(FWHM)of 46 nm,and PL quantum yield(QY)of~80%under the 470 nm excitation light.The G-CDs and corresponding composite film prepared with polyvinyl butyral(G-CDs@PVB)exhibit good PL stability after undergoing long-time storage for one year and 360 h exposure under 460 nm blue light.The G-CDs@PVB film was used as color-conversion materials in green-emitting light-emitting diode(LED)application,exhibiting a Commission internationale de l'Eclairage(CIE)chromaticity coordinate of(0.21,0.44).The film was also used in CD-based liquid crystal display(CD-LCD)application,achieving a color gamut value of 85%.This work will offer a working basis for the synthesis of high-performance CDs as well as their application in displays.

Carbon dotsOne-step synthesisNarrow bandwidthHigh quantum yieldDisplay

Rui Cheng、Tingting Zhang、Xin Huang、Jian Yu

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State Key Laboratory of Materials-Oriented Chemical Engineering,College of Chemical Engineering,Nanjing Tech University,Nanjing 210009,China

Jiangsu Funding Program for Excellent Postdoctoral Talent江苏高校优势学科建设工程项目

2022ZB369

2024

中国化学快报(英文版)
中国化学会

中国化学快报(英文版)

CSTPCD
影响因子:0.771
ISSN:1001-8417
年,卷(期):2024.35(5)
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