Recent process in developing advanced heterogeneous diatomic-site metal catalysts for electrochemical CO2 reduction

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外文摘要：Diatomic-site catalysts(DASCs)have emerged as a kind of promising heterogeneous candidate catalysts for electrochemical CO2 reduction(ECR),which is considered to retain the advantage of single-atom cat-alysts(SACs)but also introduce opportunities to exceed the limit of single-atom catalysts.In the past few years,tremendous progress has been achieved in this field.Herein,the recent progress in ECR on DASCs has been summarized.It will start with the classification of DASCs.Then the challenges in the precise fabrication and characterization of DASCs have been emphasized.By introducing the advanced ECR performance on DASCs,superior to that on SACs,the synergistic effects of the dual metal atoms are highlighted,as this origin of the advanced ECR performance on DASCs is comprehensively summa-rized.Finally,the major challenges and perspectives of DASCs have been proposed to shed light on the development of DASCs for ECR application.

外文关键词：

Diatomic-site metal catalystElectrochemical CO2 reductionClassificationCO2 activationSynergistic effects

作者：

Xueyang Zhao、Bangwei Deng、Hongtao Xie、Yizhao Li、Qingqing Ye、Fan Dong

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作者单位：

Yangtze Delta Region Institute(Huzhou),University of Electronic Science and Technology of China,Huzhou 313001,China

Institute of Fundamental and Frontier Sciences,University of Electronic Science and Technology of China,Chengdu 611731,China

Suzhou Industrial Technology Research Institute of Zhejiang University,Zhejiang University,Suzhou 215159,China

基金：

by"Pioneer"and"Leading Goose"R&D Program of ZhejiangNational Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaChina Postdoctoral Science FoundationNatural Science Foundation of Huzhou City

项目编号：

2023C030172222560622261142663221760292023M7304912022YZ22

出版年：

2024

DOI：

10.1016/j.cclet.2023.109139

中国化学快报(英文版)

中国化学会

中国化学快报(英文版)

CSTPCD

影响因子：0.771

ISSN：1001-8417

年,卷(期)：2024.35(7)