Computational simulation-assisted research on chloride solid electrolytes for lithium-ion batteries
Due to the phenomenon of easy deformation and short circuit of traditional organic liquid lithium-ion batteries,instantaneous thermal runaway occurs,resulting in combustion and even explosion.Solid-state batteries,with their excellent safety,can fundamentally solve this problem.In recent years,computational simulation has become more and more popular in the development and research of solid electrolyte,and this way of computation-assisted experiment has greatly promoted the development of electrolyte.This paper introduces the latest progress in the research of chloride electrolyte,which belongs to the category of halide electrolyte.The development process of chloride solid electrolyte is reviewed.The preparation method,modification of anion and cation regulation,optimization of structure regulation and stability of temperature,humidity and electrode material are also discussed.Finally,the problems facing the chloride solid electrolyte are summarized and analyzed,and the future development direction of the chloride solid electrolyte is further proposed.