首页|Correlating dynamic relaxation and viscoelasticity in metallic glasses

Correlating dynamic relaxation and viscoelasticity in metallic glasses

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Relaxation dynamics,essential for the structural evolution of non-equilibrium systems like glassy materials,remain enigmatic.Here,we explore relaxation dynamics and viscoelastic properties in three types of metallic glasses with distinct β relaxation behavior.In systems with significant β relaxation,stress relaxation and creep experiments reveal a transition from two-step to one-step relaxation with rising temperature.However,such a phenomenon is absent in systems with weaker β relaxation.We model the two-step relaxation process using a double Kohlrausch-Williams-Watts equation,and the obtained relaxation times elegantly adhere to the Arrhenius relationship.By combining fitted activation energies with theoretical analysis,we conclusively attribute these relaxation processes to β relaxation and α relaxation,respectively.Finally,we analyze the relaxation time spectra of two processes and establish a comprehensive picture linking dynamic relaxation with viscoelasticity.Our study provides new strategies for probing the complex relaxation behaviors of glasses from the perspective of viscoelasticity.

metallic glassesdynamics relaxationtwo-step relaxationstress relaxationcreep

GuangHui Xing、Qi Hao、Fan Zhu、Yun-Jiang Wang、Yong Yang、Hidemi Kato、Eloi Pineda、Si Lan、JiChao Qiao

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School of Mechanics,Civil Engineering and Architecture,Northwestern Polytechnical University,Xi'an 710072,China

State Key Laboratory of Nonlinear Mechanics,Institute of Mechanics,Chinese Academy of Sciences,Beijing 100190,China

School of Engineering Science,University of Chinese Academy of Sciences,Beijing 100049,China

Department of Mechanical Engineering,College of Engineering,City University of Hong Kong,Hong Kong 999077,China

Department of Materials Science and Engineering,College of Engineering,City University of Hong Kong,Hong Kong 999077,China

Institute for Materials Research,Tohoku University,Sendai 980-8577,Japan

Department of Physics,Institute of Energy Technologies,Universitat Politecnica de Catalunya,Barcelona 08019,Spain

School of Material Science and Engineering,Herbert Gleiter Institute of Nanoscience,Nanjing University of Science and Technology,Nanjing 210094,China

State Key Laboratory of Clean and Efficient Turbomachinery Power Equipment,Northwestern Polytechnical University Xi'an 710072,China

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National Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaNatural Science Basic Research Plan for Distinguished Young Scholars in Shaanxi ProvinceFundamental Research Funds for the Central UniversitiesNational Natural Science Foundation of ChinaMCIN/AEI/10.13039/501100011033Generalitat de Catalunya,AGAURNatural Science Foundation of China

51971178522711532021JC-12D500022003412072344PID2020-112975GB-I002021SGR0034352222104

2024

中国科学:物理学 力学 天文学(英文版)
中国科学院

中国科学:物理学 力学 天文学(英文版)

CSTPCD
影响因子:0.91
ISSN:1674-7348
年,卷(期):2024.67(5)