中国科学:物理学 力学 天文学(英文版)2024,Vol.67Issue(5) :109-114.DOI:10.1007/s11433-023-2327-5

Room-temperature phonon-coupled single-photon emission in hexagonal boron nitride

Jia-Min Lai Qing-Hai Tan Feilong Song Haonan Chang Yanpei Lv Xue-Lu Liu Jinghua Teng Weibo Gao Ping-Heng Tan Jun Zhang
中国科学:物理学 力学 天文学(英文版)2024,Vol.67Issue(5) :109-114.DOI:10.1007/s11433-023-2327-5

Room-temperature phonon-coupled single-photon emission in hexagonal boron nitride

Jia-Min Lai 1Qing-Hai Tan 2Feilong Song 3Haonan Chang 4Yanpei Lv 4Xue-Lu Liu 4Jinghua Teng 5Weibo Gao 6Ping-Heng Tan 4Jun Zhang4
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作者信息

  • 1. State Key Laboratory of Superlattices and Microstructures,Institute of Semiconductors,Chinese Academy of Sciences,Beijing 100083,China;Key Laboratory of Magnetic Molecules and Magnetic Information Materials of Ministry of Education & Research Institute of Materials Science,Shanxi Normal University,Taiyuan 030000,China;Center of Materials Science and Optoelectronics Engineering,University of Chinese Academy of Sciences,Beijing 100049,China
  • 2. State Key Laboratory of Superlattices and Microstructures,Institute of Semiconductors,Chinese Academy of Sciences,Beijing 100083,China;Division of Physics and Applied Physics,School of Physical and Mathematical Sciences,Nanyang Technological University,Singapore 637371,Singapore;Institute of Materials Research and Engineering(IMRE),Agency for Science,Technology and Research(A*STAR),Singapore 138634,Singapore
  • 3. State Key Laboratory of Superlattices and Microstructures,Institute of Semiconductors,Chinese Academy of Sciences,Beijing 100083,China
  • 4. State Key Laboratory of Superlattices and Microstructures,Institute of Semiconductors,Chinese Academy of Sciences,Beijing 100083,China;Center of Materials Science and Optoelectronics Engineering,University of Chinese Academy of Sciences,Beijing 100049,China
  • 5. Institute of Materials Research and Engineering(IMRE),Agency for Science,Technology and Research(A*STAR),Singapore 138634,Singapore
  • 6. Division of Physics and Applied Physics,School of Physical and Mathematical Sciences,Nanyang Technological University,Singapore 637371,Singapore
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Abstract

Photon-lattice(phonon)coupling is fundamental to light-matter interaction,particularly when it reaches the quantum limit of the phonon-coupled single-photon emission,which holds great potential for quantum manipulation and quantum information transduction.Here,we report single defect state-phonon coupling in hexagonal boron nitride(hBN)at room temperature.An ultrabroad spectrum of single-photon emissions can be achieved by selecting the excitation energies.Using photoluminescence excitation spectroscopy,we observe single-phonon-assisted resonance-enhanced single-photon emission,along with multiple phonon replicas that herald the creation of phonon Fock state.We also develop a transition model to gain insight into the physical process behind the single defect state-phonon coupling.Our work sets the stage for manipulating electron-phonon coupling state with single quantum-level precision at room temperature.

Key words

photon-phonon coupling/single-photon emission/hexagonal boron nitride

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基金项目

CAS Interdisciplinary Innovation Team()

National Natural Science Foundation of China(12074371)

Strategic Priority Research Program of Chinese Academy of Sciences(XDB28000000)

Research Equipment Development Project of Chinese Academy of Sciences(YJKYYQ20210001)

Chinese Academy of Sciencesthe Scientific and Technological Research council of TüRK?YE Joint Research Projects(172111KYSB20210004)

出版年

2024
中国科学:物理学 力学 天文学(英文版)
中国科学院

中国科学:物理学 力学 天文学(英文版)

CSTPCD
影响因子:0.91
ISSN:1674-7348
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